One-pot synthesis of C/Bi/Bi2O3 composite with enhanced photocatalytic activity

被引:162
|
作者
Hao, Qiang [1 ]
Wang, Ruiting [1 ]
Lu, Haojie [1 ]
Xie, Ci'an [1 ]
Ao, Weihua [1 ]
Chen, Daimei [1 ]
Ma, Chao [2 ]
Yao, Wenqing [2 ]
Zhu, Yongfa [2 ]
机构
[1] China Univ Geosci, Beijing Key Lab Mat Utilizat Nonmetall Minerals &, Natl Lab Mineral Mat, Sch Mat Sci & Technol, Beijing 100083, Peoples R China
[2] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
基金
中国国家自然科学基金;
关键词
Bi2O3; Plasmonic Bi metal; SPR effect; C/Bi/Bi2O3; composite; BI METAL-DEPOSITION; HETEROJUNCTION; WATER; OXIDE; DEGRADATION; REDUCTION; OXIDATION; MICROSPHERES; EFFICIENCY; TITANIUM;
D O I
10.1016/j.apcatb.2017.07.030
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this work, a novel C/Bi/Bi2O3 composite photocatalyst was prepared by a facile one -pot method, using EDTA-Bi as a precursor. The C/Bi/Bi2O3 composite photocatalyst exhibited higher photocatalytic activity than Bi2O3 on the degradation of 2,4-dichlorophenol (2,4-DCP) under both simulated sunlight and visible light irradiation. Metallic Bi and the remaining organic carbon cannot only enhance the absorption of lights, but also accelerate the seperation of photogenerated charge carriers. As a result, the photocatalytic activity is enhanced. More importantly, this paper provides a facile method for the preparation of C/Bi/Bi2O3 composite materials, which is suitable for mass production. (C) 2017 Published by Elsevier B.V.
引用
收藏
页码:63 / 72
页数:10
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