Effect of Zn/Si ratio on the microstructural and microwave dielectric properties of Zn2SiO4 ceramics

被引:110
作者
Nguyen, Ngoc-Huan
Lim, Jong-Bong
Nahm, Sahn [1 ]
Paik, Jong-Hoo
Kim, Jong-Hee
机构
[1] Korea Univ, Dept Mat Sci & Engn, Seoul 136701, South Korea
[2] Korea Inst Ceram Engn & Technol, Seoul 153801, South Korea
关键词
D O I
10.1111/j.1551-2916.2007.01891.x
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Zn2SiO4 ceramics synthesized by the conventional solid-state method exhibited a low Q x f value, possibly due to the formation of a ZnO second phase. However, with a small ZnO reduction from the Zn2SiO4 ceramics, the ZnO second phase disappeared and grain growth occurred due to the formation of a Si-rich liquid phase. Specimens with a large grain size exhibited an improved Q x f value. In particular, the ceramics with nominal composition Zn1.8SiO3.8 sintered at 1300 degrees C exhibited improved microwave dielectric properties of epsilon(r)=6.6, Q x f=147 000 GHz, and tau(f)=-22 ppm/degrees C.
引用
收藏
页码:3127 / 3130
页数:4
相关论文
共 14 条
  • [1] COURTNEY WE, 1985, IEEE T MTT, V18, P476
  • [2] Characterization and dielectric behavior of willemite and TiO2-doped willemite ceramics at millimeter-wave frequency
    Guo, YP
    Ohsato, H
    Kakimoto, KI
    [J]. JOURNAL OF THE EUROPEAN CERAMIC SOCIETY, 2006, 26 (10-11) : 1827 - 1830
  • [3] Hakki B. W., 1960, IEEE Trans. Microwave Theory Techn, V8, P402, DOI DOI 10.1109/TMTT.1960.1124749
  • [4] Hong SH, 2001, J AM CERAM SOC, V84, P1597, DOI 10.1111/j.1151-2916.2001.tb00883.x
  • [5] Microwave dielectric properties of Re3Ga5O12 (Re: Nd, Sm, Eu, Dy and Yb) ceramics and effect of TiO2 on the microwave dielectric properties of Sm3Ga5O12 ceramics
    Kim, Jae Chul
    Kim, Min-Han
    Nahm, Sahn
    Paik, Jong-Hoo
    Kim, Jong-Hee
    Lee, Hwack-Joo
    [J]. JOURNAL OF THE EUROPEAN CERAMIC SOCIETY, 2007, 27 (8-9) : 2865 - 2870
  • [6] Synthesis and microwave dielectric properties of Re3Ga5O12 (Re: Nd, Sm, Eu, Dy, Yb, and Y) ceramics
    Kim, Jae Chul
    Kim, Min-Han
    Lim, Jong-Bong
    Nahm, Sahn
    Paik, Jong-Hoo
    Kim, Jong-Hee
    [J]. JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 2007, 90 (02) : 641 - 644
  • [7] Crystal structure of corundum type Mg4(Nb2-xTax)O9 microwave dielectric ceramics with low dielectric loss
    Ogawa, H
    Kan, A
    Ishihara, S
    Higashida, Y
    [J]. JOURNAL OF THE EUROPEAN CERAMIC SOCIETY, 2003, 23 (14) : 2485 - 2488
  • [8] Controlled temperature coefficient of resonant frequency of Al2O3-TiO2 ceramics by annealing treatment
    Ohishi, Y
    Miyauchi, Y
    Ohsato, H
    Kakimoto, K
    [J]. JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 2004, 43 (6A): : L749 - L751
  • [9] Microwave-millimeterwave dielectric materials
    Ohsato, H
    Tsunooka, T
    Kan, A
    Ohishi, Y
    Miyauchi, Y
    Tohdo, Y
    Kawai, T
    Kakimoto, K
    Ogawa, H
    [J]. ELECTROCERAMICS IN JAPAN VII, 2004, 269 : 195 - 198
  • [10] Ohsato H., 2003, J. Korean Ceram. Soc., V40, P350