Efficient Formaldehyde Elimination Over Ag/MnO2 Nanorods: Influence of the Ag Loading

被引：17

作者：

Huang, Fenglin ^{[1
]}

Wang, Xue ^{[1
]}

Zhu, Qinyu ^{[1
]}

Li, Kelun ^{[2
]}

Zhou, Xuefeng ^{[1
]}

Lu, Suhong ^{[1
]}

Fan, Zheng ^{[1
]}

He, Lulu ^{[1
]}

Liu, Yanxiong ^{[1
]}

Pang, Fanjue ^{[1
]}

机构：

[1] Xian Shiyou Univ, Coll Chem & Chem Engn, Xian 710065, Shaanxi, Peoples R China

[2] Shaanxi Coal & Chem Technol Inst Co Ltd, Xian 710070, Shaanxi, Peoples R China

来源：

CATALYSIS SURVEYS FROM ASIA | 2019年 / 23卷 / 01期

关键词：

Formaldehyde; Catalytic oxidation; Ag; Nanorod; MnO2; ROOM-TEMPERATURE OXIDATION; CATALYTIC-OXIDATION; OXIDE CATALYSTS; PERFORMANCE; CO; MNO2; NANOPARTICLES; NANOSHEETS; PT/TIO2; SIO2;

D O I：

10.1007/s10563-018-9257-2

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A series of Ag/MnO2 nanorods with various loading amounts of Ag were fabricated and used for formaldehyde (HCHO) elimination. The obtained catalysts were characterized by means of N-2 adsorption-desorption, SEM, TEM, XRD, H-2-TPR, O-2-TPD and XPS. As the optimal loading amount of Ag was 0.1%, the Ag/MnO2-r exhibited a superior catalytic performance for HCHO oxidation, on which the 100% conversion of HCHO was achieved at 80 degrees C. It has observed that the remarkable catalytic activity of 0.1% Ag/MnO2-r was mainly due to the better low-temperature reducibility and more abundant surface active oxygen species resulting from the strong metal-support interaction between Ag and MnO2.

引用

页码：33 / 40

页数：8

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