Experimental observation of percolation-enhanced nonlinear light scattering from semicontinuous metal films -: art. no. 125106

被引:56
作者
Breit, M [1 ]
Podolskiy, VA
Grésillon, S
von Plessen, G
Feldmann, J
Rivoal, JC
Gadenne, P
Sarychev, AK
Shalaev, VM
机构
[1] Univ Munich, Dept Phys, Photon & Optoelect Grp, D-80799 Munich, Germany
[2] Univ Munich, CeNS, D-80799 Munich, Germany
[3] Ecole Super Phys & Chim Ind Ville Paris, Lab Opt Phys, CNRS, UPR5, F-75231 Paris, France
[4] Univ Paris 06, F-75231 Paris, France
[5] New Mexico State Univ, Dept Phys, Las Cruces, NM 88003 USA
[6] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA
[7] Univ Versailles, CNRS, UMR 8634, LMOV, F-78035 Versailles, France
关键词
D O I
10.1103/PhysRevB.64.125106
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Strongly enhanced second-harmonic generation (SHG), which is characterized by a nearly isotropic intensity distribution, is observed for gold-glass films near the percolation threshold. The diffuselike SHG scattering, which can be thought of as nonlinear critical opalescence, is in sharp contrast with highly collimated linear reflection and transmission from these nanostructured semicontinuous metal films. Our observations, which can be explained by giant fluctuations of local nonlinear sources for SHG due to plasmon localization, verify recent predictions of percolation-enhanced nonlinear scattering.
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页数:5
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共 18 条
  • [1] SURFACE-ENHANCED 2ND-HARMONIC GENERATION IN C-60-COATED SILVER ISLAND FILMS
    AKTSIPETROV, OA
    KELLER, O
    PEDERSEN, K
    NIKULIN, AA
    NOVIKOVA, NN
    FEDYANIN, AA
    [J]. PHYSICS LETTERS A, 1993, 179 (02) : 149 - 153
  • [2] PHYSICAL-PROPERTIES OF MACROSCOPICALLY INHOMOGENEOUS-MEDIA
    BERGMAN, DJ
    STROUD, D
    [J]. SOLID STATE PHYSICS: ADVANCES IN RESEARCH AND APPLICATIONS, VOL 46, 1992, 46 : 147 - 269
  • [3] OPTICAL SECOND-HARMONIC GENERATION IN REFLECTION FROM MEDIA WITH INVERSION SYMMETRY
    BLOEMBERGEN, N
    CHANG, RK
    JHA, SS
    LEE, CH
    [J]. PHYSICAL REVIEW, 1968, 174 (03): : 813 - +
  • [4] Giant field fluctuations and anomalous light scattering from semicontinuous metal films
    Brouers, F
    Blacher, S
    Sarychev, AK
    [J]. PHYSICAL REVIEW B, 1998, 58 (23) : 15897 - 15903
  • [5] SURFACE-ENCHANCED 2ND-HARMONIC GENERATION
    CHEN, CK
    DECASTRO, ARB
    SHEN, YR
    [J]. PHYSICAL REVIEW LETTERS, 1981, 46 (02) : 145 - 148
  • [6] Percolation and fractal composites:: Optical studies
    Ducourtieux, S
    Grésillon, S
    Boccara, AC
    Rivoal, JC
    Quelin, X
    Gadenne, P
    Drachev, VP
    Bragg, WD
    Safonov, VP
    Podolskiy, VA
    Ying, ZC
    Armstrong, RL
    Shalaev, VM
    [J]. JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS, 2000, 9 (01): : 105 - 116
  • [7] Giant Stokes fields on semicontinuous metal films
    Gadenne, P
    Brouers, F
    Shalaev, VM
    Sarychev, AK
    [J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1998, 15 (01) : 68 - 72
  • [8] TRANSMITTANCE AND REFLECTANCE INSITU MEASUREMENTS OF SEMICONTINUOUS GOLD-FILMS DURING DEPOSITION
    GADENNE, P
    YAGIL, Y
    DEUTSCHER, G
    [J]. JOURNAL OF APPLIED PHYSICS, 1989, 66 (07) : 3019 - 3025
  • [9] Experimental observation of localized optical excitations in random metal-dielectric films
    Grésillon, S
    Aigouy, L
    Boccara, AC
    Rivoal, JC
    Quelin, X
    Desmarest, C
    Gadenne, P
    Shubin, VA
    Sarychev, AK
    Shalaev, VM
    [J]. PHYSICAL REVIEW LETTERS, 1999, 82 (22) : 4520 - 4523
  • [10] DIFFUSELY SCATTERED 2ND-HARMONIC GENERATION FROM A SILVER FILM DUE TO SURFACE-PLASMONS
    KUANG, LP
    SIMON, HJ
    [J]. PHYSICS LETTERS A, 1995, 197 (03) : 257 - 261