Origins of suspended particulate matter based on sterol distribution in low salinity water mass observed in the offshore East China Sea

被引:17
作者
Kim, Moonkoo [1 ]
Jung, Jee-hyun [1 ]
Jin, Yongnu [1 ]
Han, Gi Myeong [1 ]
Lee, Taehee [2 ]
Hong, Sang Hee [1 ]
Yim, Un Hyuk [1 ]
Shim, Won Joon [1 ]
Choi, Dong-Lim [3 ]
Kannan, Narayanan [1 ,4 ]
机构
[1] Korea Inst Ocean Sci & Technol, Oil & POPs Res Grp, 41 Jangmok 1 Gil, Geoje 53201, South Korea
[2] Korea Inst Ocean Sci & Technol, Jeju Int Marine Sci Res & Educ Ctr, 2670 Iljudong Ro, Jeju 63349, South Korea
[3] Korea Inst Ocean Sci & Technol, South Sea Environm Res Ctr, 41 Jangmok 1 Gil, Geoje 53201, South Korea
[4] Univ Putra Malaysia, Fac Environm Studies, Upm Serdang 43400, Selangor Darul, Malaysia
关键词
Sterols; Suspended particulate matter; East China Sea; Lipid biomarkers; River plume ecosystem; ORGANIC-COMPOUNDS PRESENT; SEWAGE CONTAMINATION; FECAL STEROLS; GAS-CHROMATOGRAPHY; LIPID BIOMARKERS; CHESAPEAKE BAY; WASTE-WATER; FATTY-ACID; RIVER; ESTUARY;
D O I
10.1016/j.marpolbul.2016.04.049
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The molecular composition and distribution of sterols were investigated in the East China Sea to identify the origins of suspended particulate matter (SPM) in offshore waters influenced by Changjiang River Diluted Water (CRDW). Total sterol concentrations ranged from 3200 to 31,900 pg L-1 and 663 to 5690 pg L-1 in the particulate and dissolved phases, respectively. Marine sterols dominated representing 71% and 66% in the particulate and dissolved phases, respectively. Typical sewage markers, such as coprostanol, were usually absent at 250 km offshore. However, sterols from allochthonous terrestrial plants were still detected at these sites. A negative relationship was observed between salinity and concentrations of terrestrial sterols in SPM, suggesting that significant amounts of terrestrial particulate matter traveled long distance offshore in the East China Sea, and the Changjiang River Diluted Water (CRDW) was an effective carrier of land-derived particulate organic matter to the offshore East China Sea. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:281 / 288
页数:8
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