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Photocatalytic degradation of C.I. Basic Violet 10 using TiO2 catalysts supported by Y zeolite:: An investigation of the effects of operational parameters
被引:222
作者:
Wang, Cheng-Cai
[1
]
Lee, Chung-Kung
Lyu, Meng-Du
Juang, Lain-Chuen
机构:
[1] Vanung Univ, Green Environm R&D Ctr, Tao Yuan 32061, Taiwan
[2] Vanung Univ, Dept Environm Engn, Tao Yuan 32061, Taiwan
关键词:
TiO2;
Y zeolite;
photocatalytic degradation;
cationic dye;
operational parameters;
catalyst;
D O I:
10.1016/j.dyepig.2007.02.004
中图分类号:
O69 [应用化学];
学科分类号:
081704 ;
摘要:
The physical and chemical states of zeolite-supported TiO2 were evaluated via powder X-ray diffraction (XRD), Fourier transform infrared (FTIR) and nitrogen adsorption-desorption isotherms. The effects of operational parameters, including TiO2 content, calcination temperature, pH, initial dye concentration, as well as catalyst dosage, on photocatalytic degradation performance were examined. The photocatalytic reaction followed first-order kinetics for all catalysts; optimum photodegradation efficiency was found to result from the use of a high TiO2 concentration (20% TiO2), a calcination temperature of 600 degrees C, alkaline pH (9-10) and a catalyst dosage of 5333 ppm. (c) 2007 Elsevier Ltd. All rights reserved.
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页码:817 / 824
页数:8
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