Electromagnetic Shielding by MXene-Graphene-PVDF Composite with Hydrophobic, Lightweight and Flexible Graphene Coated Fabric

被引:94
作者
Raagulan, Kanthasamy [1 ]
Braveenth, Ramanaskanda [1 ]
Jang, Hee Jung [1 ]
Lee, Yun Seon [2 ]
Yang, Cheol-Min [2 ]
Kim, Bo Mi [3 ]
Moon, Jai Jung [4 ]
Chai, Kyu Yun [1 ]
机构
[1] Wonkwang Univ, Div Bionanochem, Coll Nat Sci, Iksan 570749, South Korea
[2] Korea Inst Sci & Technol, Multifunct Struct Composite Res Ctr, Inst Adv Composite Mat, Chudong Ro 92, Wanju Gun 55324, Jeollabukdo, South Korea
[3] Wonkwang Univ, Dept Chem Engn, Iksan 570749, South Korea
[4] Clean & Sci Co Ltd, Jeongeup 3 Ind Complex 15BL,67,3Sandan 3 Gil, Buk Myeon 56136, Jeongeup Si, South Korea
基金
新加坡国家研究基金会;
关键词
graphene; MXene; EMI shielding; composite; fabric; WALLED CARBON NANOTUBES; HIGH-PERFORMANCE; ELECTROCHEMICAL PERFORMANCE; TI3C2TX MXENE; OXIDE; CARBIDE; NANOCOMPOSITES; FIBER; FILM; NANOPARTICLES;
D O I
10.3390/ma11101803
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
MXene and graphene based thin, flexible and low-density composite were prepared by cost effective spray coating and solvent casting method. The fabricated composite was characterized using Raman spectroscopy, X-ray diffraction (XRD), scanning electron microscope (SEM), X-ray photoelectron spectroscopy (XPS) and energy dispersive X-ray (EDX). The prepared composites showed hydrophobic nature with higher contact angle of 126 degrees, -43 mNm(-1) wetting energy, -116 mNm(-1) spreading Coefficient and 30 mNm(-1) lowest work of adhesion. The composites displayed excellent conductivity of 13.68 Scm(-1) with 3.1 sq(-1) lowest sheet resistance. All the composites showed an outstanding thermal stability and constrain highest weight lost until 400 degrees C. The MXene-graphene foam exhibited excellent EMI shielding of 53.8 dB (99.999%) with reflection of 13.10 dB and absorption of 43.38 dB in 8-12.4 GHz. The single coated carbon fabric displayed outstanding absolute shielding effectiveness of 35,369.82 dBcm(2)g(-1). The above results lead perspective applications such as aeronautics, radars, air travels, mobile phones, handy electronics and military applications.
引用
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页数:19
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