Orientational control of pentacene crystals on SiO2 by graphoepitaxy to improve lateral carrier transport

被引:5
|
作者
Li, Shi-Guang [1 ,2 ]
Nakayama, Naoki [2 ]
Sakai, Masatoshi [2 ]
Kudo, Kazuhiro [2 ]
Matsubara, Ryosuke [1 ]
Nakamura, Masakazu [1 ]
机构
[1] Nara Inst Sci & Technol, Grad Sch Mat Sci, Nara 6300192, Japan
[2] Chiba Univ, Dept Elect & Elect Engn, Inage Ku, Chiba 2638522, Japan
关键词
Organic thin-film transistors; Pentacene; Graphoepitaxy; Grain boundaries; Periodic grooves; ORGANIC TRANSISTORS; THIN-FILM; INTERFACE; CRYSTALLIZATION; GRATINGS;
D O I
10.1016/j.orgel.2012.01.027
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We controlled the in-plane orientation of pentacene grains by graphoepitaxy using patterned amorphous-SiO2/Si substrates on which periodic grooves with slope edges had been formed. Pentacene crystals exhibited a clear tendency to align their b-axes perpendicular to the groove edges. Organic thin-film transistors were fabricated on the patterned and flat substrates and their transistor characteristics were compared. Although the patterned substrates increased the apparent mobility by only 10-20%, the number of grain boundaries with high potential barriers to carrier transport was reduced to half of that on flat substrates. This improvement is expected to enhance the response speed of pentacene organic thin-film transistors and suppress the sensitivity of their characteristics to the operating temperature. (C) 2012 Elsevier B. V. All rights reserved.
引用
收藏
页码:864 / 869
页数:6
相关论文
共 50 条
  • [21] Interface and Carrier Transport Behaviour in Al/HfO2/SiO2/SiC Structure
    Mahapatra, R.
    Horsfall, A. B.
    Wright, N. G.
    SILICON CARBIDE AND RELATED MATERIALS 2007, PTS 1 AND 2, 2009, 600-603 : 759 - 762
  • [22] Enhancement of carrier mobility in pentacene thin-film transistor on SiO2 by controlling the initial film growth modes
    Qi, Qiong
    Yu, Aifang
    Jiang, Peng
    Jiang, Chao
    APPLIED SURFACE SCIENCE, 2009, 255 (09) : 5096 - 5099
  • [23] Carrier transport in high-efficiency ZnO/SiO2/Si solar cells
    Wenas, Wilson W.
    Riyadi, Syarif
    SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2006, 90 (18-19) : 3261 - 3267
  • [24] Vertical charge-carrier transport in Si nanocrystal/SiO2 multilayer structures
    Osinniy, V.
    Lysgaard, S.
    Kolkovsky, Vl
    Pankratov, V.
    Larsen, A. Nylandsted
    NANOTECHNOLOGY, 2009, 20 (19)
  • [25] Theoretical prediction of universal curves for carrier transport in Si/SiO2(100) interfaces
    Ishihara, Takamitsu
    Kato, Koichi
    JOURNAL OF APPLIED PHYSICS, 2013, 114 (05)
  • [26] Electroluminescence and carrier transport of SiO2 film containing different density of Ge nanocrystals
    Department of Physics, Nanjing Normal University, Nanjing 210097, China
    Appl Phys Lett, 17 (2459-2461):
  • [28] Electroluminescence and carrier transport of SiO2 film containing different density of Ge nanocrystals
    Zhang, JY
    Ye, YH
    Tan, XL
    APPLIED PHYSICS LETTERS, 1999, 74 (17) : 2459 - 2461
  • [29] Modification of the electric conduction at the pentacene/SiO2 interface by surface termination of SiO2 -: art. no. 103502
    Yagi, I
    Tsukagoshi, K
    Aoyagi, Y
    APPLIED PHYSICS LETTERS, 2005, 86 (10) : 1 - 3
  • [30] Hot-carrier injections in SiO2
    Vuillaume, D
    Bravaix, A
    Goguenheim, D
    MICROELECTRONICS RELIABILITY, 1998, 38 (01) : 7 - 22