Fischer-Tropsch Synthesis over Molecular Sieve Supported Catalysts

被引：68

作者：

Sun, Bo ^{[1
,2
]}

Qiao, Minghua ^{[1
,2
]}

Fan, Kangnian ^{[1
,2
]}

Ulrich, Jeffrey ^{[3
]}

Tao, Franklin ^{[4
]}

机构：

[1] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China

[2] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China

[3] Univ Notre Dame, Dept Chem & Biomol Engn, Notre Dame, IN 46556 USA

[4] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA

来源：

CHEMCATCHEM | 2011年 / 3卷 / 03期

基金：

美国国家科学基金会;

关键词：

cracking; Fischer-Tropsch; hydrogenation; isomerization; syngas; CARBON-MONOXIDE HYDROGENATION; HIGHLY DISPERSED PALLADIUM; CO HYDROGENATION; COBALT CATALYSTS; IRON CATALYSTS; ISO-PARAFFINS; SYNTHESIS GAS; MOSSBAUER-SPECTROSCOPY; BIMETALLIC CATALYSTS; MESOPOROUS MATERIALS;

D O I：

10.1002/cctc.201000352

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

For sustainable fuel production from alternative energy sources, it is important to design and develop Fischer-Tropsch synthesis (FTS) catalysts for hydrocarbons that deviate from the Anderson-Schulz-Flory distribution. The introduction of a molecular sieve to a conventional FTS catalyst system offers the opportunity to confine spatially the chain length of the hydro-carbons, and to convert long-chain hydrocarbons to molecules more suitable as transportation fuels. The incorporation of metal nanoparticles in a variety of molecular sieves with different methods allows a versatile means to modulate the distribution of the FTS hydrocarbons for different purposes.

引用

页码：542 / 550

页数：9

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