Atmospheric pressure glow discharge for CO2 conversion: Model-based exploration of the optimum reactor configuration

被引:54
作者
Trenchev, G. [1 ]
Nikiforov, A. [2 ]
Wang, W. [1 ]
Kolev, St. [3 ]
Bogaerts, A. [1 ]
机构
[1] Univ Antwerp, Res Grp PLASMANT, Dept Chem, Univ Pl 1, B-2610 Antwerp, Belgium
[2] Univ Ghent, Dept Appl Phys, St Pietersnieuwstr 41, B-9000 Ghent, Belgium
[3] Sofia Univ, Fac Phys, 5 James Bourchier Blvd, Sofia 1164, Bulgaria
关键词
Plasma; CO2; conversion; Atmospheric; Glow discharge; Vortex flow; Modeling; PLASMA;
D O I
10.1016/j.cej.2019.01.091
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We investigate the performance of an atmospheric pressure glow discharge (APGD) reactor for CO2 conversion in three different configurations, through experiments and simulations. The first (basic) configuration utilizes the well-known pin-to-plate design, which offers a limited conversion. The second configuration improves the reactor performance by employing a vortex-flow generator. The third, "confined" configuration is a complete redesign of the reactor, which encloses the discharge in a limited volume, significantly surpassing the conversion rate of the other two designs. The plasma properties are investigated using an advanced plasma model.
引用
收藏
页码:830 / 841
页数:12
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