Single Atom Excels as the Smallest Functional Material

被引:123
作者
Zhang, Wei [1 ,2 ,3 ,4 ]
Zheng, Weitao [1 ,2 ,3 ,5 ]
机构
[1] Jilin Univ, Dept Mat Sci, Changchun 130012, Peoples R China
[2] Jilin Univ, Key Lab Mobile Mat MOE, Changchun 130012, Peoples R China
[3] Jilin Univ, State Key Lab Automot Simulat & Control, Changchun 130012, Peoples R China
[4] CIC Energigune, Parque Tecnol Alava, Albert Einstein 48, Ed Cic Minano 01510, Spain
[5] Ikerbasque, Basque Fdn Sci, E-48011 Bilbao, Spain
关键词
NITROGEN-DOPED GRAPHENE; WATER-GAS SHIFT; CO OXIDATION; ELECTRON-MICROSCOPY; SOLID CATALYSTS; SPECTROSCOPY; LAYER; SITE; CONFINEMENT; PERFORMANCE;
D O I
10.1002/adfm.201600240
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The emerging single-atom field spans single-atom catalysis in chemistry and single-atom manipulation in physics up to the state-of-the-art characterization via imaging and spectroscopy. These interdisciplinary progresses have been interacted closely with the development of materials science, underscoring the principle that the single atom excels as the smallest functional material. This simple concept not only permits to reinvent our understanding of the nature of materials, but also promises unambiguously to have a great impact on other physical sciences.
引用
收藏
页码:2988 / 2993
页数:6
相关论文
共 98 条
  • [21] Graphene: Status and Prospects
    Geim, A. K.
    [J]. SCIENCE, 2009, 324 (5934) : 1530 - 1534
  • [22] Rh1/-Al2O3 Single-Atom Catalysis of O2 Activation and CO Oxidation: Mechanism, Effects of Hydration, Oxidation State, and Cluster Size
    Ghosh, Tushar K.
    Nair, Nisanth N.
    [J]. CHEMCATCHEM, 2013, 5 (07) : 1811 - 1821
  • [23] Direct, Nonoxidative Conversion of Methane to Ethylene, Aromatics, and Hydrogen
    Guo, Xiaoguang
    Fang, Guangzong
    Li, Gang
    Ma, Hao
    Fan, Hongjun
    Yu, Liang
    Ma, Chao
    Wu, Xing
    Deng, Dehui
    Wei, Mingming
    Tan, Dali
    Si, Rui
    Zhang, Shuo
    Li, Jianqi
    Sun, Litao
    Tang, Zichao
    Pan, Xiulian
    Bao, Xinhe
    [J]. SCIENCE, 2014, 344 (6184) : 616 - 619
  • [24] Atomic-scale structure of single-layer MoS2 nanoclusters
    Helveg, S
    Lauritsen, JV
    Lægsgaard, E
    Stensgaard, I
    Norskov, JK
    Clausen, BS
    Topsoe, H
    Besenbacher, F
    [J]. PHYSICAL REVIEW LETTERS, 2000, 84 (05) : 951 - 954
  • [25] Electronic Metal- Support Interactions in Single- Atom Catalysts
    Hu, Pingping
    Huang, Zhiwei
    Amghouz, Zakariae
    Makkee, Michiel
    Xu, Fei
    Kapteijn, Freek
    Dikhtiarenko, Alla
    Chen, Yaxin
    Gu, Xiao
    Tang, Xingfu
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2014, 53 (13) : 3418 - 3421
  • [26] Three-Dimensional Imaging of Individual Dopant Atoms in SrTiO3
    Hwang, Jinwoo
    Zhang, Jack Y.
    D'Alfonso, Adrian J.
    Allen, Leslie J.
    Stemmer, Susanne
    [J]. PHYSICAL REVIEW LETTERS, 2013, 111 (26)
  • [27] Inducing Magnetism in Pure Organic Molecules by Single Magnetic Atom Doping
    Iancu, Violeta
    Braun, Kai-Felix
    Schouteden, Koen
    Van Haesendonck, Chris
    [J]. PHYSICAL REVIEW LETTERS, 2014, 113 (10)
  • [29] Direct observation of defect-mediated cluster nucleation
    Kaiser, U
    Muller, DA
    Grazul, JL
    Chuvilin, A
    Kawasaki, M
    [J]. NATURE MATERIALS, 2002, 1 (02) : 102 - 105
  • [30] Detection of single atoms and buried defects in three dimensions by aberration-corrected electron microscope with 0.5-Å information limit
    Kisielowski, C.
    Freitag, B.
    Bischoff, M.
    van Lin, H.
    Lazar, S.
    Knippels, G.
    Tiemeijer, P.
    van der Stam, M.
    von Harrach, S.
    Stekelenburg, M.
    Haider, M.
    Uhlemann, S.
    Mueller, H.
    Hartel, P.
    Kabius, B.
    Miller, D.
    Petrov, I.
    Olson, E. A.
    Donchev, T.
    Kenik, E. A.
    Lupini, A. R.
    Bentley, J.
    Pennycook, S. J.
    Anderson, I. M.
    Minor, A. M.
    Schmid, A. K.
    Duden, T.
    Radmilovic, V.
    Ramasse, Q. M.
    Watanabe, M.
    Erni, R.
    Stach, E. A.
    Denes, P.
    Dahmen, U.
    [J]. MICROSCOPY AND MICROANALYSIS, 2008, 14 (05) : 469 - 477