Graphene Near-Degenerate Four-Wave Mixing for Phase Characterization of Broadband Pulses in Ultrafast Microscopy

被引：29

作者：

Ciesielski, Richard ^{[1
,2
]}

Comin, Alberto ^{[1
,2
]}

Handloser, Matthias ^{[1
,2
]}

Donkers, Kevin ^{[1
,2
]}

Piredda, Giovanni ^{[3
]}

Lombardo, Antonio ^{[4
]}

Ferrari, Andrea C. ^{[4
]}

Hartschuh, Achim ^{[1
,2
]}

机构：

[1] Univ Munich, Dept Chem, Butenandtstr 5-13, D-81377 Munich, Germany

[2] Univ Munich, CeNS, D-81377 Munich, Germany

[3] Fachhsch Vorarlberg, Josef Ressel Zentrum, A-6850 Dornbirn, Austria

[4] Univ Cambridge, Cambridge Graphene Ctr, Cambridge CB3 0FA, England

来源：

NANO LETTERS | 2015年 / 15卷 / 08期

基金：

英国工程与自然科学研究理事会; 欧洲研究理事会;

关键词：

Graphene; four-wave mixing; pulse shaping femtosecond laser; microscopy; phase retrieval; MULTIPHOTON INTRAPULSE INTERFERENCE; ULTRASHORT LASER-PULSES;

D O I：

10.1021/acs.nanolett.5b00893

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We investigate near-degenerate four-wave mixing in graphene using femtosecond laser pulse shaping microscopy. Intense near-degenerate four-wave mixing signals on either side of the exciting laser spectrum are controlled by amplitude and phase shaping. Quantitative signal modeling for the input pulse parameters shows a spectrally flat phase response of the near-degenerate four-wave mixing due to the linear dispersion of the massless Dirac Fermions in graphene. Exploiting these properties we demonstrate that graphene is uniquely suited for the intrafocus phase characterization and compression of broadband laser pulses, circumventing disadvantages of common methods utilizing second or third harmonic light.

引用

页码：4968 / 4972

页数：5

共 34 条

[1] Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles [J].

Accanto, Nicolo ;

Nieder, Jana B. ;

Piatkowski, Lukasz ;

Castro-Lopez, Marta ;

Pastorelli, Francesco ;

Brinks, Daan ;

van Hulst, Niek F. .

LIGHT-SCIENCE & APPLICATIONS, 2014, 3 :e143-e143

[2]

[Anonymous], 2006, Nonlinear Optics

[3]

Bonaccorso F, 2010, NAT PHOTONICS, V4, P611, DOI [10.1038/nphoton.2010.186, 10.1038/NPHOTON.2010.186]

[4] Polar Fe(IO3)3 nanocrystals as local probes for nonlinear microscopy [J].

Bonacina, L. ;

Mugnier, Y. ;

Courvoisier, F. ;

Le Dantec, R. ;

Extermann, J. ;

Lambert, Y. ;

Boutou, V. ;

Galez, C. ;

Wolf, J.-P. .

APPLIED PHYSICS B-LASERS AND OPTICS, 2007, 87 (03) :399-403

[5] Compression of ultrashort laser pulses via gated multiphoton intrapulse interference phase scans [J].

Comin, Alberto ;

Ciesielski, Richard ;

Piredda, Giovanni ;

Donkers, Kevin ;

Hartschuh, Achim .

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2014, 31 (05) :1118-1125

[6] Science and technology roadmap for graphene, related two-dimensional crystals, and hybrid systems [J].

Ferrari, Andrea C. ;

Bonaccorso, Francesco ;

Fal'ko, Vladimir ;

Novoselov, Konstantin S. ;

Roche, Stephan ;

Boggild, Peter ;

Borini, Stefano ;

Koppens, Frank H. L. ;

Palermo, Vincenzo ;

Pugno, Nicola ;

Garrido, Jose A. ;

Sordan, Roman ;

Bianco, Alberto ;

Ballerini, Laura ;

Prato, Maurizio ;

Lidorikis, Elefterios ;

Kivioja, Jani ;

Marinelli, Claudio ;

Ryhaenen, Tapani ;

Morpurgo, Alberto ;

Coleman, Jonathan N. ;

Nicolosi, Valeria ;

Colombo, Luigi ;

Fert, Albert ;

Garcia-Hernandez, Mar ;

Bachtold, Adrian ;

Schneider, Gregory F. ;

Guinea, Francisco ;

Dekker, Cees ;

Barbone, Matteo ;

Sun, Zhipei ;

Galiotis, Costas ;

Grigorenko, Alexander N. ;

Konstantatos, Gerasimos ;

Kis, Andras ;

Katsnelson, Mikhail ;

Vandersypen, Lieven ;

Loiseau, Annick ;

Morandi, Vittorio ;

Neumaier, Daniel ;

Treossi, Emanuele ;

Pellegrini, Vittorio ;

Polini, Marco ;

Tredicucci, Alessandro ;

Williams, Gareth M. ;

Hong, Byung Hee ;

Ahn, Jong-Hyun ;

Kim, Jong Min ;

Zirath, Herbert ;

van Wees, Bart J. .

NANOSCALE, 2015, 7 (11) :4598-4810

[7] The rise of graphene [J].

Geim, A. K. ;

Novoselov, K. S. .

NATURE MATERIALS, 2007, 6 (03) :183-191

[8] Controllable optical negative refraction and phase conjugation in graphite thin films [J].

Harutyunyan, Hayk ;

Beams, Ryan ;

Novotny, Lukas .

NATURE PHYSICS, 2013, 9 (07) :423-425

[9] Coherent Nonlinear Optical Response of Graphene [J].

Hendry, E. ;

Hale, P. J. ;

Moger, J. ;

Savchenko, A. K. ;

Mikhailov, S. A. .

PHYSICAL REVIEW LETTERS, 2010, 105 (09)

[10]

Koppens FHL, 2014, NAT NANOTECHNOL, V9, P780, DOI [10.1038/NNANO.2014.215, 10.1038/nnano.2014.215]

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