Regeneration Behavior of a Sustainable Bioinspired Soybean-Based Solvent for CO2 Capture

被引:4
作者
Gusnawan, Pri J. [1 ]
Zou, Lusi [1 ]
Zhang, Guoyin [1 ]
Yu, Jianjia [1 ]
机构
[1] New Mexico Inst Min & Technol, Petr Recovery Res Ctr, Socorro, NM 87801 USA
来源
ACS SUSTAINABLE CHEMISTRY & ENGINEERING | 2020年 / 8卷 / 09期
关键词
CO2; capture; SBB solvent; Amino acid; Regeneration behavior; Energy consumption; CO2-LOADED MEA SOLUTION; AMINO-ACID-COMPOSITION; ENERGY REQUIREMENT; ABSORPTION; DESORPTION; MONOETHANOLAMINE; REDUCTION; KINETICS; SINGLE; SALT;
D O I
10.1021/acssuschemeng.9b07689
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The high-energy penalty for CO, capture is mainly attributed to the energy consumption for the regeneration of CO2-loaded solvent. In this study, a bioinspired soybean-based solvent (SBB solvent) was prepared according to the composition of amino acid in the commercially available hydrolyzed soy protein, which contains 18 different amino acids with the pH ranging from 13 (arginine) to 4.5 (aspartic acid) in the potassium hydroxide solution. The regeneration behavior of the SBB solvent was investigated in batch experiments under different operating conditions. The regeneration performance of the SBB solvent was evaluated in terms of CO2 desorption rate, CO2 desorption efficiency, and specific energy consumption. The result showed that the regeneration behavior of the SBB solvent was highly determined by the heating source temperature, initial CO2 loading, and solvent concentration. Compared to the conventional monoethanolamine, the SBB solvent proved to have 205% more CO2 desorption efficiency, up to 195% faster CO2 desorption rate, and 37% lower specific regeneration energy. The SBB solvent possesses great potential as new sustainable solvents for energy-efficient CO2 capture in the future.
引用
收藏
页码:3929 / 3937
页数:17
相关论文
共 36 条
  • [1] [Anonymous], 2018, INTRO CHEM ENG THERM
  • [2] [Anonymous], 2018, HDB PHASE CHANGE BOI
  • [3] Reduction of Energy Requirement of CO2 Desorption by Adding Acid into CO2-Loaded Solvent
    Feng, Bo
    Du, Min
    Dennis, Timothy James
    Anthony, Kim
    Perumal, Marc Jarrod
    [J]. ENERGY & FUELS, 2010, 24 (01) : 213 - 219
  • [4] Hydrolysis and amino acid composition analysis of proteins
    Fountoulakis, M
    Lahm, HW
    [J]. JOURNAL OF CHROMATOGRAPHY A, 1998, 826 (02) : 109 - 134
  • [5] Corrosion and degradation in MEA based post-combustion CO2 capture
    Fytianos, Georgios
    Ucar, Seniz
    Grimstvedt, Andreas
    Hyldbakk, Astrid
    Svendsen, Hallvard F.
    Knuutila, Hanna K.
    [J]. INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2016, 46 : 48 - 56
  • [6] Experimental research on the performance of CO2-loaded solutions of MEA and DEA at regeneration conditions
    Galindo, Paula
    Schaeffer, Anke
    Brechtel, Kevin
    Unterberger, Sven
    Scheffknecht, Guenter
    [J]. FUEL, 2012, 101 : 2 - 8
  • [7] Geankoplis C. J., 2013, Transport processes and separation process principles, V4th ed.
  • [8] Performance and stability of a bio-inspired soybean-based solvent for CO2 capture from flue gas
    Gusnawan, Pri J.
    Zou, Lusi
    Zhang, Guoyin
    Yu, Jianjia
    [J]. CHEMICAL ENGINEERING JOURNAL, 2020, 385
  • [9] Soybean and moringa based green biosolvents for low-concentration CO2 capture via a hollow fiber membrane contactor
    Gusnawan, Pri Januar
    Zha, Shangwen
    Zou, Lusi
    Zhang, Guoyin
    Yu, Jianjia
    [J]. CHEMICAL ENGINEERING JOURNAL, 2018, 335 : 631 - 637
  • [10] Liquid Speciation Study in Amine Amino Acid Salts for CO2 Absorbent with 13C-NMR
    Hartono, A.
    Aronu, U. E.
    Svendsen, H. F.
    [J]. 10TH INTERNATIONAL CONFERENCE ON GREENHOUSE GAS CONTROL TECHNOLOGIES, 2011, 4 : 209 - 215