Extraction-Dominated Temperature Degradation of Population Inversion in Terahertz Quantum Cascade Lasers

被引:3
作者
Wu, Yuyang [1 ]
Zhang, Jinchuan [2 ]
Zhao, Yunhao [1 ]
Liang, Chongyun [3 ]
Liu, Fengqi [2 ]
Shi, Yi [4 ,5 ]
Che, Renchao [1 ,6 ]
机构
[1] Fudan Univ, Dept Mat Sci, Shanghai Key Lab Mol Catalysis & Innovat Mat, Lab Adv Mat, Shanghai 200438, Peoples R China
[2] Chinese Acad Sci, Beijing Key Lab Low Dimens Semicond Mat & Devices, Inst Semicond, Key Lab Semicond Mat Sci, Beijing 100083, Peoples R China
[3] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China
[4] Nanjing Univ, Sch Elect Sci & Engn, Natl Lab Solid State Microstruct, Nanjing 210093, Peoples R China
[5] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China
[6] Zhejiang Lab, Joint Res Ctr Computat Mat, Hangzhou 311100, Peoples R China
基金
中国国家自然科学基金;
关键词
extraction efficiency; phonon scattering; population inversion; temperature degradation; terahertz quantum cascade lasers; SCATTERING;
D O I
10.1002/smll.202106943
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Degraded population inversion (PI) at elevated temperature, regarded as an important temperature degradation factor in terahertz quantum cascade lasers (THz QCL), has hindered the widespread use of these devices. Herein, the mechanism of the temperature degradation of PI is investigated microscopically. It is demonstrated that the limited extraction efficiency of the extraction system dominates the decrease of PI at elevated temperatures. To be specific, the increased temperature brings about intense thermally activated longitudinal optical phonon scattering, leading to large amounts of electrons scattering to lower level state. In this case, the resonant-phonon extraction system is incapable of depleting all the electrons from lower level states. So even though the resonant-tunneling injection seems efficient enough to compensate the electron runoff at the upper state, the electron density at lower level state increases and the overall PI turns out lower. In addition, it is found that strong electron-ionized donor separation at high temperature can induce level misalignment, which can stagger the optimal conditions of injection and extraction. Also, the extraction efficiency gets lower as the extraction system requires accurate coupling between several energy levels.
引用
收藏
页数:8
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