Composition of a gas and ash mixture formed during the pyrolysis and combustion of coal-water slurries containing petrochemicals

被引:43
作者
Dorokhov, V. V. [1 ]
Kuznetsov, G., V [1 ]
Nyashina, G. S. [1 ]
Strizhak, P. A. [1 ]
机构
[1] Natl Res Tomsk Polytech Univ, 30 Lenin Ave, Tomsk 634050, Russia
关键词
Coal-water slurries; Petrochemicals; Pyrolysis; Combustion; Anthropogenic emissions; Relative performance indicator; SULFUR TRANSFORMATION; POLLUTANT EMISSIONS; PULVERIZED COAL; TRACE-ELEMENTS; SEWAGE-SLUDGE; BIOMASS; COCOMBUSTION; BEHAVIOR; FUEL; WASTE;
D O I
10.1016/j.envpol.2021.117390
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This paper presents the results of experimental research into the component composition of gases and ash residue from the combustion of a set of high-potential coal-water slurries containing petrochemicals. We have established that the use of slurry fuels provides a decrease in the CO2, CH4, SO2, and NOx concentrations as compared to those from coal combustion. The content of carbon monoxide and hydrogen in the gas environment from the combustion of slurries is higher due to the intense water evaporation. It is shown that adding biomass allows a further 5-33% reduction in the emissions of nitrogen and sulfur oxides as compared to the coal-water slurry and the composition with added waste turbine oil and a 23-68% decrease as compared to coal (per unit mass of the fuel burnt). The mechanisms and stages of CO2, SO2, and NOx formation are explained with a view to controlling gaseous anthropogenic emissions and ash buildup. The values of the relative environmental performance indicator are calculated for slurry fuels. It is shown to exceed the same indicator of bituminous coal by 28-56%.
引用
收藏
页数:14
相关论文
共 73 条
[1]   Comparative analysis of factors affecting differences in the concentrations of gaseous anthropogenic emissions from coal and slurry fuel combustion [J].
Akhmetshin, M. R. ;
Nyashina, G. S. ;
Strizhak, P. A. .
FUEL, 2020, 270
[2]  
[Anonymous], 2013, D368213 ASTM INT
[3]   Co-combustion of coal and olive oil industry residues in fluidised bed [J].
Armesto, L ;
Bahillo, A ;
Cabanillas, A ;
Veijonen, K ;
Otero, J ;
Plumed, A ;
Salvador, L .
FUEL, 2003, 82 (08) :993-1000
[4]   Fuel additive technology - NOx reduction, combustion efficiency and fly ash improvement for coal fired power stations [J].
Daood, S. S. ;
Ord, G. ;
Wilkinson, T. ;
Nimmo, W. .
FUEL, 2014, 134 :293-306
[5]   Sustainable Management and Action in China under the Increasing Risks of Global Climate Change [J].
Ding, Yihui .
ENGINEERING, 2018, 4 (03) :301-305
[6]   Field-based emission measurements of biomass burning in typical Chinese built-in-place stoves [J].
Du, Wei ;
Zhu, Xi ;
Chen, Yuanchen ;
Liu, Weijian ;
Wang, Wei ;
Shen, Guofeng ;
Tao, Shu ;
Jetter, James J. .
ENVIRONMENTAL POLLUTION, 2018, 242 :1587-1597
[7]   Intensity dependent features of the light-induced gasification of the waste-derived coal-water compositions [J].
Egorov, Roman I. ;
Zaitsev, Alexander S. ;
Li, Hong ;
Gao, Xin ;
Strizhak, Pavel A. .
RENEWABLE ENERGY, 2020, 146 :1667-1675
[8]   An effective recycle way of waste coke ash and coking wastewater for preparing coke ash coking wastewater slurry [J].
Fan, Yaoyao ;
Wang, Ruixin ;
Sun, Jinyan ;
Xiang, Jin ;
Wang, Ruiqi ;
Sun, Huanwu .
SCIENCE OF THE TOTAL ENVIRONMENT, 2020, 742
[9]   Structural changes of global power generation capacity towards sustainability and the risk of stranded investments supported by a sustainability indicator [J].
Farfan, Javier ;
Breyer, Christian .
JOURNAL OF CLEANER PRODUCTION, 2017, 141 :370-384
[10]   Sulphur retention during co-combustion of coal and sewage sludge [J].
Folgueras, MB ;
Díaz, RM ;
Xiberta, J .
FUEL, 2004, 83 (10) :1315-1322