Synergistic Effect of Dual Ligands on Stable Blue Quasi-2D Perovskite Light-Emitting Diodes

被引:139
作者
Jin, Yan [1 ]
Wang, Zhao-Kui [1 ]
Yuan, Shuai [1 ]
Wang, Qiang [1 ]
Qin, Chaochao [2 ]
Wang, Kai-Li [1 ]
Dong, Chong [1 ]
Li, Meng [1 ]
Liu, Yufang [2 ]
Liao, Liang-Sheng [1 ]
机构
[1] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Peoples R China
[2] Henan Normal Univ, Henan Key Lab Infrared Mat & Spectrum Measures &, Xinxiang 453007, Henan, Peoples R China
基金
国家重点研发计划;
关键词
ligand synergistic effect; perovskite light-emitting diodes; stable blue spectra; MIXED HALIDE PEROVSKITES;
D O I
10.1002/adfm.201908339
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Since the emergence of inorganic-organic hybrid perovskites a few years ago, there have been many promising achievements in the field of green and red perovskite light-emitting diodes (PeLEDs). Nevertheless, the performance of blue-light PeLEDs faces challenges. In this work, the unique synergy obtained by introducing two different ligands to successfully form quasi-2D perovskite films, which can exhibit stable blue-light emission, is utilized. The fabricated PeLEDs have a maximum external quantum efficiency of 2.62% and a half lifetime (T-50) of 8.8 min. Meanwhile, the electroluminescence spectrum with its peak located at 485 nm, demonstrates improved stability by applying different voltage bias. The finding in this work offers a new way to achieve steady blue PeLEDs with high performance.
引用
收藏
页数:6
相关论文
共 27 条
[1]   Perovskite light-emitting diodes based on spontaneously formed submicrometre-scale structures [J].
Cao, Yu ;
Wang, Nana ;
Tian, He ;
Guo, Jingshu ;
Wei, Yingqiang ;
Chen, Hong ;
Miao, Yanfeng ;
Zou, Wei ;
Pan, Kang ;
He, Yarong ;
Cao, Hui ;
Ke, You ;
Xu, Mengmeng ;
Wang, Ying ;
Yang, Ming ;
Du, Kai ;
Fu, Zewu ;
Kong, Decheng ;
Dai, Daoxin ;
Jin, Yizheng ;
Li, Gongqiang ;
Li, Hai ;
Peng, Qiming ;
Wang, Jianpu ;
Huang, Wei .
NATURE, 2018, 562 (7726) :249-+
[2]   High-Performance Color-Tunable Perovskite Light Emitting Devices through Structural Modulation from Bulk to Layered Film [J].
Chen, Ziming ;
Zhang, Chongyang ;
Jiang, Xiao-Fang ;
Liu, Meiyue ;
Xia, Ruoxi ;
Shi, Tingting ;
Chen, Dongcheng ;
Xue, Qifan ;
Zhao, Yu-Jun ;
Su, Shijian ;
Yip, Hin-Lap ;
Cao, Yong .
ADVANCED MATERIALS, 2017, 29 (08)
[3]   Sky-blue perovskite light-emitting diodes based on quasi-two-dimensional layered perovskites [J].
Cheng, Lu ;
Cao, Yu ;
Ge, Rui ;
Wei, Ying-Qiang ;
Wang, Na-Na ;
Wang, Jian-Pu ;
Huang, Wei .
CHINESE CHEMICAL LETTERS, 2017, 28 (01) :29-31
[4]   Anion-exchange red perovskite quantum dots with ammonium iodine salts for highly efficient light-emitting devices [J].
Chiba, Takayuki ;
Hayashi, Yukihiro ;
Ebe, Hinako ;
Hoshi, Keigo ;
Sato, Jun ;
Sato, Shugo ;
Pu, Yong-Jin ;
Ohisa, Satoru ;
Kido, Junji .
NATURE PHOTONICS, 2018, 12 (11) :681-+
[5]   Tunable Light-Emitting Diodes Utilizing Quantum-Confined Layered Perovskite Emitters [J].
Congreve, Daniel N. ;
Weidman, Mark C. ;
Seitz, Michael ;
Paritmongkol, Watcharaphol ;
Dahod, Nabeel S. ;
Tisdale, William A. .
ACS PHOTONICS, 2017, 4 (03) :476-481
[6]   2D Ruddlesden-Popper Perovskite Nanoplate Based Deep-Blue Light-Emitting Diodes for Light Communication [J].
Deng, Wei ;
Jin, Xiangcheng ;
Lv, You ;
Zhang, Xiujuan ;
Zhang, Xiaohong ;
Jie, Jiansheng .
ADVANCED FUNCTIONAL MATERIALS, 2019, 29 (40)
[7]   Rationalizing the light-induced phase separation of mixed halide organic-inorganic perovskites [J].
Draguta, Sergiu ;
Sharia, Onise ;
Yoon, Seog Joon ;
Brennan, Michael C. ;
Morozov, Yurii V. ;
Manser, Joseph M. ;
Kamat, Prashant V. ;
Schneider, William F. ;
Kuno, Masaru .
NATURE COMMUNICATIONS, 2017, 8
[8]   Reversible photo-induced trap formation in mixed-halide hybrid perovskites for photovoltaics [J].
Hoke, Eric T. ;
Slotcavage, Daniel J. ;
Dohner, Emma R. ;
Bowring, Andrea R. ;
Karunadasa, Hemamala I. ;
McGehee, Michael D. .
CHEMICAL SCIENCE, 2015, 6 (01) :613-617
[9]   Identifying and Reducing Interfacial Losses to Enhance Color-Pure Electroluminescence in Blue-Emitting Perovskite Nanoplatelet Light-Emitting Diodes [J].
Hoye, Robert L. Z. ;
Lai, May-Ling ;
Anaya, Miguel ;
Tong, Yu ;
Galkowski, Krzysztof ;
Doherty, Tiarnan ;
Li, Weiwei ;
Huq, Tahmida N. ;
Mackowski, Sebastian ;
Polavarapu, Lakshminarayana ;
Feldmann, Jochen ;
MacManus-Driscoll, Judith L. ;
Friend, Richard H. ;
Urban, Alexander S. ;
Stranks, Samuel D. .
ACS ENERGY LETTERS, 2019, 4 (05) :1181-1188
[10]   Surface passivation of perovskite film for efficient solar cells [J].
Jiang, Qi ;
Zhao, Yang ;
Zhang, Xingwang ;
Yang, Xiaolei ;
Chen, Yong ;
Chu, Zema ;
Ye, Qiufeng ;
Li, Xingxing ;
Yin, Zhigang ;
You, Jingbi .
NATURE PHOTONICS, 2019, 13 (07) :460-+