Forensic signatures from laser isotope separation

被引:3
作者
Burns, Henry S. [1 ]
Biegalski, Steven R. [1 ]
机构
[1] Georgia Inst Technol, Nucl & Radiol Engn, 770 State St NW, Atlanta, GA 30313 USA
关键词
Atomic vapor laser isotope separation; Uranium enrichment; Nonproliferation; Minor isotopes; Uranium isotope ratios; ENRICHMENT;
D O I
10.1007/s10967-022-08516-6
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
This work introduces an analysis of the Atomic Vapor Laser Isotope Separation (AVLIS) process to assist regulatory agencies in detecting and inspecting uranium AVLIS facilities. Operating parameters of a theoretical AVLIS device are calculated based on product and tails assays. Further analysis shows a direct relationship between feed assays of minor isotopes and product assays, allowing inspectors to confirm the method of a sample's enrichment and identify the feedstock origin due to natural variations in U-234 assay. The decay of U-234 into Th-230 is used to estimate the time of last enrichment and increase the accuracy of feed assay calculations.
引用
收藏
页码:4947 / 4952
页数:6
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