Synthesis and Characterisation of Porous Titania-Silica Composite Aerogel for NOx and Acetaldehyde Removal

被引:11
作者
Lee, Kwang Young [1 ,2 ]
Park, Se Min [1 ,2 ]
Kim, Jong Beom [1 ,2 ]
El Saliby, Ibrahim [3 ]
Shahid, Mohammad [3 ]
Kim, Geon-Joong [4 ]
Shon, Ho Kyong [3 ]
Kim, Jong-Ho [1 ,2 ]
机构
[1] Chonnam Natl Univ, Sch Appl Chem Engn, Gwangju 500757, South Korea
[2] Chonnam Natl Univ, Res Inst Catalysis, Gwangju 500757, South Korea
[3] UTS, Fac Engn & Informat Technol, POB 123, Broadway, NSW 2007, Australia
[4] Inha Univ, Dept Chem Engn, Inchon 402751, South Korea
基金
新加坡国家研究基金会; 澳大利亚研究理事会;
关键词
Titania; Photocatalysis; Silica; Acetaldehyde; NOx; SOL-GEL SYNTHESIS; SUPERHYDROPHOBIC SILICA; SURFACE MODIFICATION; PHYSICAL-PROPERTIES; AMBIENT-PRESSURE; MIXED OXIDES; TIO2-SIO2; WATER; NANOPARTICLES; PERFORMANCE;
D O I
10.1166/jnn.2016.10997
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this study, the synthesis of porous titania-silica (TiO2-SiO2) composite aerogel at ambient pressure by using non-hazardous chemicals as a source of silica was investigated. TiO2-SiO2 composite aerogels were characterised and their photocatalytic performances were investigated for the removal efficiency of acetaldehyde and NOx under UV light. Results showed that porous composite aerogel with aggregated morphology, high surface area and an increased mesoporosity were formed. TiO2-SiO2(1.8) composite, with high Ti/Si ratio, showed the best results in terms of photocatalytic removal of acetaldehyde and nitrogen oxide.
引用
收藏
页码:4505 / 4511
页数:7
相关论文
共 24 条
[1]   Elaboration and characterization of TiO2 nanoparticles incorporated in SiO2 host matrix [J].
Amlouk, A. ;
El Mir, L. ;
Kraiem, S. ;
Alaya, S. .
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 2006, 67 (07) :1464-1468
[2]   Superhydrophobic silica aerogel powders with simultaneous surface modification, solvent exchange and sodium ion removal from hydrogels [J].
Bhagat, Sharad D. ;
Kim, Yong-Ha ;
Suh, Kuen-Hack ;
Ahn, Young-Soo ;
Yeo, Jeong-Gu ;
Han, Jong-Hun .
MICROPOROUS AND MESOPOROUS MATERIALS, 2008, 112 (1-3) :504-509
[3]   Sol-Gel Synthesis of Inorganic Mesostructured Composite Photocatalyst for Water Purification: An Insight Into the Synthesis Fundamentals, Reaction, and Binding Mechanisms [J].
Chong, Meng Nan ;
Jin, Bo .
SYNTHESIS AND REACTIVITY IN INORGANIC METAL-ORGANIC AND NANO-METAL CHEMISTRY, 2012, 42 (01) :68-75
[4]   Effects of H2O2 pretreatment on surface characteristics and bioactivity of NaOH-treated NiTi shape memory alloy [J].
Chu Cheng-lin ;
Hu Tao ;
Zhou Jun ;
Pu Yue-pu ;
Yin Li-Hong ;
Dong Yin-sheng ;
Lin Ping-hua ;
Chung Jonathan-C Y ;
Chu Paul-K .
TRANSACTIONS OF NONFERROUS METALS SOCIETY OF CHINA, 2006, 16 (06) :1295-1300
[5]   Silica aerogel; synthesis, properties and characterization [J].
Dorcheh, A. Soleimani ;
Abbasi, M. H. .
JOURNAL OF MATERIALS PROCESSING TECHNOLOGY, 2008, 199 (1-3) :10-26
[6]   Synthesis, characterisation and performance of (TiO2)0.18(SiO2)0.82 xerogel catalysts [J].
Holland, MA ;
Pickup, DM ;
Mountjoy, G ;
Tsang, ESC ;
Wallidge, GW ;
Newport, RJ ;
Smith, ME .
JOURNAL OF MATERIALS CHEMISTRY, 2000, 10 (11) :2495-2501
[7]   Antimicrobial nanomaterials for water disinfection and microbial control: Potential applications and implications [J].
Li, Qilin ;
Mahendra, Shaily ;
Lyon, Delina Y. ;
Brunet, Lena ;
Liga, Michael V. ;
Li, Dong ;
Alvarez, Pedro J. J. .
WATER RESEARCH, 2008, 42 (18) :4591-4602
[8]   Hydrothermal synthesis, characterization, and photocatalytic performance of silica-modified titanium dioxide nanoparticles [J].
Li, ZJ ;
Hou, B ;
Xu, Y ;
Wu, D ;
Sun, YH .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2005, 288 (01) :149-154
[9]   Comparative study of sol-gel-hydrothermal and sol-gel synthesis of titania-silica composite nanoparticles [J].
Li, ZJ ;
Hou, B ;
Xu, Y ;
Wu, D ;
Sun, YH ;
Hu, W ;
Deng, F .
JOURNAL OF SOLID STATE CHEMISTRY, 2005, 178 (05) :1395-1405
[10]  
Liu Hui, 2009, Chinese Journal of Pathology, V38, P347, DOI 10.3760/cma.j.issn.0529-5807.2009.05.016