Advanced treatment of coal gasification wastewater by O3/Fenton in a rotating packed bed in tandem with coagulation

被引:9
作者
Ma, Huapeng [1 ]
Zhao, Zemeng [2 ]
Shi, Yuanteng [2 ]
Xiao, Hao [1 ]
Han, Rong [1 ]
Wang, Lei [1 ]
Shao, Lei [1 ]
机构
[1] Beijing Univ Chem Technol, Res Ctr, Minist Educ High Grav Engn & Technol, Beijing 100029, Peoples R China
[2] China Coal Energy Res Inst Co Ltd, Clean Utilizat Res Inst, Xian 710054, Shanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
Coal gasification wastewater; Ozone; Fenton; Rotating packed bed; Mass transfer; Coagulation; HETEROGENEOUS FENTON OXIDATION; ACTIVATED CARBON; ELECTRO-FENTON; REMOVAL; OZONE; INTEGRATION; OZONATION; DEGRADATION; ABSORPTION; MECHANISM;
D O I
10.1016/j.cep.2021.108664
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
In this study, the O-3/Fenton system in a rotating packed bed (RPB) in tandem with coagulation process was applied to the advanced treatment of coal gasification wastewater (CGW). The removal of COD reached 35.4% in the O-3/Fenton@RPB process, and the total removal of COD rose to 47.8% after the effluent of the O-3/Fenton@RPB process was further treated with coagulation. The O-3/Fenton@RPB + coagulation tandem process also demonstrates good effect on enhancing biodegradation and removing color of the CGW, with the BOD5/COD and decolorization in the tandem process reaching 0.49 and 87.5%, respectively. In addition, an artificial neural network model was established to predict the mass transfer performance of the O-3/Fenton system in the RPB and exhibited a good predictability. The O-3/Fenton@RPB + coagulation tandem process shows the application potential in the advanced treatment of CGW.
引用
收藏
页数:8
相关论文
共 42 条
  • [1] Synthesis of nano-fibers of aluminum hydroxide in novel rotating packed bed reactor
    Chen, JF
    Shao, L
    Guo, F
    Wang, XM
    [J]. CHEMICAL ENGINEERING SCIENCE, 2003, 58 (3-6) : 569 - 575
  • [2] Two-stage air stripping combined with hydrolysis acidification process for coal gasification wastewater pretreatment
    Chen, Xiurong
    Sun, Xiaoli
    Wang, Xiaoxiao
    Xu, Peng
    Yang, Chenchen
    Lu, Quanling
    Wang, Shanshan
    [J]. WATER SCIENCE AND TECHNOLOGY, 2019, 79 (11) : 2185 - 2194
  • [3] Investigation of hydrolysis acidification process during anaerobic treatment of coal gasification wastewater (CGW): Evolution of dissolved organic matter and biotoxicity
    Chen, Zhiqiang
    Li, Da
    Wen, Qinxue
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2020, 723
  • [4] Biodegradability of slaughterhouse wastewater with high blood content under anaerobic and aerobic conditions
    del Pozo, R
    Tas, DO
    Dulkadiroglu, H
    Orhon, D
    Diez, V
    [J]. JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY, 2003, 78 (04) : 384 - 391
  • [5] Dennett KE, 1996, J AM WATER WORKS ASS, V88, P129
  • [6] An investigation on the optimal location of ozonation within biological treatment for a tannery wastewater
    Dogruel, Serdar
    Genceli, Esra A.
    Babuna, Fatos G.
    Orhon, Derin
    [J]. JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY, 2006, 81 (12) : 1877 - 1885
  • [7] Edzwald JK, 1999, WATER SCI TECHNOL, V40, P63, DOI 10.2166/wst.1999.0444
  • [8] Treatment of Acid Red 73 wastewater by the O3/RSR-BCR process
    Fan, Jinmeng
    Fan, Fei
    Wang, Wei
    Zhang, Hanxiao
    Wang, Lei
    Chang, Jiawei
    Liang, Qi
    Wang, Dan
    Liu, Zhibang
    Shao, Lei
    [J]. CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2021, 160
  • [9] A comparison of spent resin degradation by Fenton and O3-Fenton process
    Feng, Wendong
    Li, Jian
    Gao, Kai
    An, Hongxiang
    Wang, Yunhai
    [J]. PROGRESS IN NUCLEAR ENERGY, 2020, 130
  • [10] Heat integration of phenols and ammonia recovery process for the treatment of coal gasification wastewater
    Gai, Hengjun
    Feng, Yirong
    Lin, Kaiqiang
    Guo, Kai
    Xiao, Meng
    Song, Hongbing
    Chen, Xiaolu
    Zhou, Hua
    [J]. CHEMICAL ENGINEERING JOURNAL, 2017, 327 : 1093 - 1101