Significantly reduced leakage currents in organic thin film transistors with Mn-doped Bi2Ti2O7 high-k gate dielectrics

被引:6
作者
Cho, Kwang-Hwan [2 ]
Kang, Min-Gyu [1 ]
Jang, Ho Won [1 ]
Shin, Hyun Yong [3 ]
Kang, Chong-Yun [1 ]
Yoon, Seok-Jin [1 ]
机构
[1] Korea Adv Inst Sci & Technol, Elect Mat Res Ctr, Seoul 130650, South Korea
[2] Univ Wisconsin, Dept Mat Sci, Madison, WI 53706 USA
[3] Namseoul Univ, Dept Elect Engn, Cheonan 331707, South Korea
来源
PHYSICA STATUS SOLIDI-RAPID RESEARCH LETTERS | 2012年 / 6卷 / 05期
关键词
OTFT; high-k gate dielectrics; BiTiO; leakage currents; PULSED-LASER DEPOSITION; CHEMICAL SOLUTION DECOMPOSITION; ELECTRICAL-PROPERTIES; STRONTIUM-TITANATE; INSULATORS;
D O I
10.1002/pssr.201206080
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report the fabrication of organic thin-film transistors (OTFTs) with high-k gate dielectrics of Mn-doped Bi2Ti2O7 (BTO) films. 3% Mn-doped BTO films deposited on polymer substrates by pulsed laser deposition at room temperature exhibit low leakage currents of 2.1 x 10(8) A/cm2 at an applied electric field of 0.3 MV/cm, while undoped BTO films show much higher leakage currents of 4.3 x 10(4) A/cm2. Mn doping effectively reduces the number of oxygen vacancies in the films and improves the electrical properties. Low operation voltage and significantly reduced leakage currents are demonstrated in pentacene-based OTFTs with the Mn-doped BTO gate dielectrics. (C) 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
引用
收藏
页码:208 / 210
页数:3
相关论文
共 17 条
[1]   Solution-Processable Barium Titanate and Strontium Titanate Nanoparticle Dielectrics for Low-Voltage Organic Thin-Film Transistors [J].
Cai, Qin Jia ;
Gan, Ye ;
Chan-Park, Mary B. ;
Yang, Hong Bin ;
Lu, Zhi Song ;
Li, Chang Ming ;
Guo, Jun ;
Dong, Zhi Li .
CHEMISTRY OF MATERIALS, 2009, 21 (14) :3153-3161
[2]   Effect of oxygen vacancies on the electrical properties of Bi6Ti5TeO22 thin film [J].
Choi, Chang-Hak ;
Choi, Joo-Young ;
Cho, Kyung-Hoon ;
Yoo, Myong-Jae ;
Nahm, Sahn ;
Kang, Chong-Yun ;
Yoon, Seok-Jin ;
Kim, Jong-Hee .
ELECTROCHEMICAL AND SOLID STATE LETTERS, 2008, 11 (11) :G51-G54
[3]   Oxygen pressure and Mn-doping effects on the structure and leakage current of Bi6Ti5TeO22 thin film [J].
Choi, Chang-Hak ;
Choi, Joo-Young ;
Cho, Kyung-Hoon ;
Yoo, Myong-Jae ;
Nahm, Sahn ;
Kang, Chong-Yun ;
Yoon, Seok-Jin ;
Kim, Jong-Hee .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2008, 155 (10) :G199-G202
[4]   Effect of oxygen vacancy and Mn-doping on electrical properties of Bi4Ti3O12 thin film grown by pulsed laser deposition [J].
Choi, Joo-Young ;
Choi, Chang-Hak ;
Cho, Kyung-Hoon ;
Seong, Tae-Geun ;
Nahm, Sahn ;
Kang, Chong-Yun ;
Yoon, Seok-Jin ;
Kim, Jong-Hee .
ACTA MATERIALIA, 2009, 57 (08) :2454-2460
[5]  
Dimitrakopoulos CD, 2002, ADV MATER, V14, P99, DOI 10.1002/1521-4095(20020116)14:2<99::AID-ADMA99>3.0.CO
[6]  
2-9
[7]   Low-voltage organic transistors on plastic comprising high-dielectric constant gate insulators [J].
Dimitrakopoulos, CD ;
Purushothaman, S ;
Kymissis, J ;
Callegari, A ;
Shaw, JM .
SCIENCE, 1999, 283 (5403) :822-824
[8]   Synthesis and structural study of stoichiometric BiTi2O7 pyrochlore [J].
Hector, AL ;
Wiggin, SB .
JOURNAL OF SOLID STATE CHEMISTRY, 2004, 177 (01) :139-145
[9]   Mn-doped Ba0.6Sr0.4TiO3 high-K gate dielectrics for low voltage organic transistor on polymer substrate -: art. no. 242908 [J].
Kang, KT ;
Lim, MH ;
Kim, HG ;
Choi, Y ;
Tuller, HL ;
Kim, ID ;
Hong, JM .
APPLIED PHYSICS LETTERS, 2005, 87 (24) :1-3
[10]   Room temperature fabricated ZnO thin film transistor using high-K Bi1.5Zn1.0Nb1.5O7 gate insulator prepared by sputtering [J].
Kim, Il-Doo ;
Lim, Mi-Hwa ;
Kang, KyongTae ;
Kim, Ho-Gi ;
Choi, Si-Young .
APPLIED PHYSICS LETTERS, 2006, 89 (02)