Organic persistent toxic substances in soils, waters and sediments along an altitudinal gradient at Mt. Sagarmatha, Himalayas, Nepal

被引:80
作者
Guzzella, Licia [1 ]
Poma, Giulia [1 ]
De Paolis, Adolfo [1 ]
Roscioli, Claudio [1 ]
Viviano, Gaetano [1 ]
机构
[1] IRSA CNR, I-20047 Brugherio, MB, Italy
关键词
PTSs; Himalayas; Sediment; Soil; Lake water; POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; POLYCHLORINATED-BIPHENYLS PCBS; EVEREST NATIONAL-PARK; MOUNTAIN LAKE WATERS; ORGANOCHLORINE COMPOUNDS; HISTORICAL MAPS; ANDEAN LAKES; RIVER-BASIN; ARCTIC LAKE;
D O I
10.1016/j.envpol.2011.06.015
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Persistent Organic Pollutants (POPS) and Polycyclic Aromatic Hydrocarbons (PAHs) are important classes of compounds of serious environmental concern. These compounds were measured in waters, sediments and soils from several high altitude sites in the Sagarmatha National Park (Nepal) and included in the Himalayan ridge. In water samples, low-level substituted PCBs and PBDEs, along with more volatile PAHs, were the most common contaminants. In sediment and soil samples, the PCB profile was mainly composed of medium-level chlorinated congeners and significantly correlated with altitude. The PAH profile for water and soil samples showed the main contribution of pyrogenic PAHs due to emissions of solid combustion, whereas the profile for sediments indicated the main contribution of pyrogenic PAHs from gasoline emissions. The PAH levels measured in Himalayan samples must be considered as low to medium contaminated, whereas the regarded Himalayan stations can be considered undisturbed remote areas concerning PCB, PBDE and OC compounds. (C) 2011 Elsevier Ltd. All rights reserved.
引用
收藏
页码:2552 / 2564
页数:13
相关论文
共 69 条
[1]  
[Anonymous], IARC MON EV CARC RIS
[2]   SEDIMENT TRAP FLUXES AND BENTHIC RECYCLING OF ORGANIC-CARBON, POLYCYCLIC AROMATIC-HYDROCARBONS, AND POLYCHLOROBIPHENYL CONGENERS IN LAKE-SUPERIOR [J].
BAKER, JE ;
EISENREICH, SJ ;
EADIE, BJ .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1991, 25 (03) :500-509
[3]   Persistent toxic substances in soils and waters along an altitudinal gradient in the Laja River Basin, Central Southern Chile [J].
Barra, R ;
Popp, P ;
Quiroz, R ;
Bauer, C ;
Cid, H ;
von Tümpling, W .
CHEMOSPHERE, 2005, 58 (07) :905-915
[4]  
Barry RG., 1982, ATMOSPHERE WEATHER C
[5]   Origin and bioavailability of PAHs in the Mediterranean sea from mussel and sediment records [J].
Baumard, P ;
Budzinski, H ;
Michon, Q ;
Garrigues, P ;
Burgeot, T ;
Bellocq, J .
ESTUARINE COASTAL AND SHELF SCIENCE, 1998, 47 (01) :77-90
[6]  
BERLUNG O, 2001, ENVIRON SCI TECHNOL, V24, P342
[7]   Firewood consumption along an altitudinal gradient in mountain villages of India [J].
Bhatt, BP ;
Sachan, MS .
BIOMASS & BIOENERGY, 2004, 27 (01) :69-75
[8]   Improvements in the analysis of decabromodiphenyl ether using on-column injection and electron-capture detection [J].
Binelli, Andrea ;
Roscioli, Claudio ;
Guzzella, Licia .
JOURNAL OF CHROMATOGRAPHY A, 2006, 1136 (02) :243-247
[9]   Accumulation of persistent organochlorine compounds in mountains of western Canada [J].
Blais, JM ;
Schindler, DW ;
Muir, DCG ;
Kimpe, LE ;
Donald, DB ;
Rosenberg, B .
NATURE, 1998, 395 (6702) :585-588
[10]   Organochlorine compounds in soils and sediments of the mountain Andean Lakes [J].
Borghini, F ;
Grimalt, JO ;
Sanchez-Hernandez, JC ;
Barra, R ;
García, CJT ;
Focardi, S .
ENVIRONMENTAL POLLUTION, 2005, 136 (02) :253-266