Feasibility of destruction of gaseous benzene with dielectric barrier discharge

被引：64

作者：

Yea, Zhaolian ^{[1
,2
]}

Zhang, Yaning ^{[1
]}

Li, Ping ^{[1
]}

Yang, Longyu ^{[1
]}

Zhang, Renxi ^{[1
]}

Hou, Huiqi ^{[1
]}

机构：

[1] Fudan Univ, Inst Environm Sci, Shanghai 200433, Peoples R China

[2] Jiangsu Teachers Univ Technol, Changzhou 213001, Peoples R China

来源：

JOURNAL OF HAZARDOUS MATERIALS | 2008年 / 156卷 / 1-3期

关键词：

benzene destruction; dielectric barrier discharge; feasibility; mechanism;

D O I：

10.1016/j.jhazmat.2007.12.048

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Destruction of gaseous benzene (C6H6) by dielectric barrier discharge (DBD) was studied in both laboratory-scale and scale-up DBD systems. The effects of input power, gas flow rate as well as initial concentration on benzene decomposition and energy yield were investigated. In addition, qualitative analysis on byproducts and relatively detailed discussion on mechanisms were also presented in this paper. At last, we systematically illustrated the feasibility of benzene removal with DBD on basis of three aspects: estimation of treatment cost per unit volume, comparison with other plasmas, and problems existed in DBD system. The results will help impel actual application of DBD on waste gas containing benzene. (C) 2007 Elsevier B.V. All rights reserved.

引用

页码：356 / 364

页数：9

共 29 条

[1] Oxidation of styrene in a silent discharge plasma [J].

Anderson, GK ;

Snyder, H ;

Coogan, J .

PLASMA CHEMISTRY AND PLASMA PROCESSING, 1999, 19 (01) :131-151

[2] Phenol production in benzene/air plasmas at atmospheric pressure. Role of radical and ionic routes [J].

Ascenzi, Daniela ;

Franceschi, Pietro ;

Guella, Graziano ;

Tosi, Paolo .

JOURNAL OF PHYSICAL CHEMISTRY A, 2006, 110 (25) :7841-7847

[3]

BAI XR, 2000, PHYSICS, V29, P406

[4] On the formation of benzene oxide/oxepin in the gas-phase reaction of OH radicals with benzene [J].

Berndt, T ;

Böge, O ;

Herrmann, H .

CHEMICAL PHYSICS LETTERS, 1999, 314 (5-6) :435-442

[5] Destruction of styrene in an air stream by packed dielectric barrier discharge reactors [J].

Chang, CL ;

Bai, HL ;

Lu, SJ .

PLASMA CHEMISTRY AND PLASMA PROCESSING, 2005, 25 (06) :641-657

[6] Low-temperature plasma-catalytic oxidation of formaldehyde in atmospheric pressure gas streams [J].

Ding, Hui-Xian ;

Zhu, Ai-Min ;

Lu, Fu-Gong ;

Xu, Yong ;

Zhang, Jing ;

Yang, Xue-Feng .

JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2006, 39 (16) :3603-3608

[7] A combined plasma photolysis (CPP) method for removal Of CS2 from gas streams at atmospheric pressure [J].

Fang, Hao He ;

Hou, Hui Qi ;

Xia, Lan Yan ;

Shu, Xiao Hong ;

Zhang, Ren Xi .

CHEMOSPHERE, 2007, 69 (11) :1734-1739

[8] Synergistic effect of silent discharge plasma and catalysts on benzene decomposition [J].

Futamura, S ;

Einaga, H ;

Kabashima, H ;

Hwan, LY .

CATALYSIS TODAY, 2004, 89 (1-2) :89-95

[9]

Guo YF, 2006, J ENVIRON SCI, V18, P276

[10]

Hou J, 1999, SHANGHAI ENV SCI, V18, P151

← 1 2 3 →