III-V Semiconductor Materials for Solar Hydrogen Production: Status and Prospects

被引：70

作者：

Tournet, Julie ^{[1
]}

Lee, Yonghwan ^{[1
]}

Krishna, Siva K. ^{[1
,2
]}

Tan, Hark H. ^{[1
]}

Jagadish, Chennupati ^{[1
]}

机构：

[1] Australian Natl Univ, Dept Elect Mat Engn, Res Sch Phys, Canberra, ACT 2601, Australia

[2] Australian Natl Univ, Res Sch Elect Energy & Mat Engn, Canberra, ACT 2601, Australia

来源：

ACS ENERGY LETTERS | 2020年 / 5卷 / 02期

基金：

澳大利亚研究理事会;

关键词：

PHOTOELECTROCHEMICAL DEVICE; CONVERSION EFFICIENCY; MOLYBDENUM-DISULFIDE; HIGH-PERFORMANCE; WATER; GAN; CELLS; GENERATION; GROWTH; NANOWIRES;

D O I：

10.1021/acsenergylett.9b02582

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Following recent developments in photoelectrochemical and photovoltaic-electrosynthetic systems, we present the benefits of III-V semiconductors for solar water splitting. In addition to their interesting light absorption and carrier transport properties, III-V alloys and multijunction structures enable the highest solar-to-hydrogen conversion efficiencies. However, many obstacles still stand in the way of practical realization of III-V solar water-splitting systems. Various surface protection strategies are being developed to address the instability of III-V semiconductors in an electrolyte. Meanwhile, multiple cost-reduction approaches are being implemented, including the use of solar concentration, epitaxial lift-off or spalling for substrate reuse, and monolithic or heterogeneous integration on silicon substrates. All these advances make III-V photoabsorbers a promising route toward decarbonated hydrogen production and pave the way to long-term deployment in real-world applications.

引用

页码：611 / 622

页数：23

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