Sediment records of Sb and Pb stable isotopic ratios in Lake Qinghai

被引:10
作者
Xu, Libin [1 ]
Wu, Fengchang [1 ]
Zheng, Jian [2 ]
Xie, Qianli [3 ]
Li, Huixian [1 ]
Liao, Haiqing [1 ]
Zhao, Xiaoli [1 ]
Guo, Fei [1 ]
机构
[1] Chinese Res Inst Environm Sci, State Environm Protect Key Lab Lake Pollut Contro, Beijing 100012, Peoples R China
[2] Natl Inst Radiol Sci, Nakaminato Lab Marine Radioecol, Environm Radiat Effects Res Grp, Hitachinaka, Ibaraki 3111202, Japan
[3] Trent Univ, Worsfold Water Qual Ctr, Peterborough, ON K9H 7B8, Canada
关键词
Antimony; Sediment; Lake Qinghai; Pb isotopic ratios; OMBROTROPHIC PEAT BOG; ANTIMONY; LEAD; ENVIRONMENT;
D O I
10.1016/j.microc.2010.05.012
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
A sediment core in Lake Qinghai in northwest China was collected in 2006. Cs-137 and Pb-210 activities were analyzed to investigate the chronology of the sediment core. Sb and Pb concentrations, and Pb stable isotopic ratios were analyzed to study the historical atmospheric deposition records and sources of Sb over the past 15 centuries. The Sb concentration was 4.21 +/- 1.52 mu g/g in the sediments, its vertical distribution of Sb shows three large peaks in the recent two centuries, 1799, 1896 and 1944, coincided with Sb contamination from large wars, respectively. The peak in 1920 responded the large earthquake that happened in northern China, which was not far away from Lake Qinghai. The Sb/Pb ratio, Pb-206/Pb-207 and Pb-208/Pb-206 results suggest that Sb and Pb were probably from the ores in South China and coals in North China before 1965, but obviously from uses of leaded gasoline after 1965. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:25 / 29
页数:5
相关论文
共 31 条
[1]   Antimony sinks in the weathering crust of bullets from Swiss shooting ranges [J].
Ackermann, Sonia ;
Giere, Reto ;
Newville, Matthew ;
Majzlan, Juraj .
SCIENCE OF THE TOTAL ENVIRONMENT, 2009, 407 (05) :1669-1682
[2]  
Appleby P.G., 1978, Catena, V5, P1, DOI [10.1016/S0341-8162(78)80002-2, DOI 10.1016/S0341-8162(78)80002-2]
[3]   A comparison of antimony and lead profiles over the past 2500 years in Flanders Moss ombrotrophic peat bog, Scotland [J].
Cloy, JM ;
Farmer, JG ;
Graham, MC ;
MacKenzie, AB ;
Cook, GT .
JOURNAL OF ENVIRONMENTAL MONITORING, 2005, 7 (12) :1137-1147
[4]   Antimony availability in highly polluted soils and sediments - A comparison of single extractions [J].
Ettler, Vojtech ;
Mihaljevic, Martin ;
Sebek, Ondrej ;
Nechutny, Zbysek .
CHEMOSPHERE, 2007, 68 (03) :455-463
[5]   Antimony in the environment: a review focused on natural waters I. Occurrence [J].
Filella, M ;
Belzile, N ;
Chen, YW .
EARTH-SCIENCE REVIEWS, 2002, 57 (1-2) :125-176
[6]   PHYSIOLOGY OF METAL TOXICITY IN PLANTS [J].
FOY, CD ;
CHANEY, RL ;
WHITE, MC .
ANNUAL REVIEW OF PLANT PHYSIOLOGY AND PLANT MOLECULAR BIOLOGY, 1978, 29 :511-566
[7]  
[高志友 GAO Zhiyou], 2005, [广东微量元素科学, Guangdong Weiliang Yuansu Kexue], V12, P17
[8]   Arsenic and antimony: comparative approach on mechanistic toxicology [J].
Gebel, T .
CHEMICO-BIOLOGICAL INTERACTIONS, 1997, 107 (03) :131-144
[9]   Historical pollution of seldom monitored trace elements in Sweden -: Part B:: Sediment analysis of silver, antimony, thallium and indium [J].
Grahn, E. ;
Karlsson, S. ;
Karlsson, U. ;
Duker, A. .
JOURNAL OF ENVIRONMENTAL MONITORING, 2006, 8 (07) :732-744
[10]  
Gurnani Neelam, 1994, Nucleus (Calcutta), V37, P71