Study on TiO2/g-C3N4 S-Scheme heterojunction photocatalyst for enhanced formaldehyde decomposition

被引:21
|
作者
Wu, Yihai [1 ]
Meng, Deqin [2 ,3 ]
Guo, Qingbin [2 ]
Gao, Dengzheng [2 ]
Wang, Li [2 ]
机构
[1] Shandong Univ Sci & Technol, Coll Safety & Environm Engn, Qingdao 266590, Peoples R China
[2] Shandong Univ Sci & Technol, Coll Chem & Biol Engn, Qingdao 266590, Peoples R China
[3] Qingdao Geoengn Survering Inst, Qingdao Geol Explorat Dev Bur, Qingdao 266000, Peoples R China
关键词
Graphitic carbon nitride; Photocatalysis; S-Scheme heterojunction; HCHO; CARBON NITRIDE G-C3N4; GASEOUS FORMALDEHYDE; DEGRADATION; COMPOSITE; NANOPARTICLES; PERFORMANCE; OXIDATION; REDUCTION; CATALYST; KINETICS;
D O I
10.1016/j.optmat.2022.112213
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Photocatalytic degradation of pollutants is one of the most environmentally friendly and energy efficient technologies. Photocatalysts with porous structures not only enhance the adsorption of pollutants by the catalyst, but also accelerate the electron transfer and enhance the photocatalytic performance due to the exposure of more active sites. In addition, the S-Scheme heterojunction photocatalyst not only reduces the rate of electron-hole pair compounding, but also maintains the redox properties of the photocatalyst and improves photocatalytic performance. In this paper, the mesoporous material TiO2/g-C3N4 S-Scheme heterojunction photocatalysts were prepared in one step by the sol-gel method using urea as a precursor. The particles of the prepared nanomaterials are between 20 and 50 nm in size and uniformly dispersed. The photodegradation efficiency of the photocatalyst for formaldehyde under visible light can reach over 85%. One-step preparation of TiO2/g-C3N4 photocatalysts by sol-gel method with simple preparation method and high yield, solving the difficulties of low yield and high requirements for temperature and environmental conditions in the preparation of g-C3N4 using urea thermal polymerisation.
引用
收藏
页数:8
相关论文
共 50 条
  • [1] Study on TiO2/g-C3N4 S-Scheme heterojunction photocatalyst for enhanced formaldehyde decomposition
    Wu, Yihai
    Meng, Deqin
    Guo, Qingbin
    Gao, Dengzheng
    Wang, Li
    Optical Materials, 2022, 126
  • [2] g-C3N4/TiO2 S-scheme heterojunction photocatalyst with enhanced photocatalytic Carbamazepine degradation and mineralization
    Kane, Abdoulaye
    Chafiq, Latifa
    Dalhatou, Sadou
    Bonnet, Pierre
    Nasr, Maryline
    Gaillard, Nathalie
    Dikdim, Jean Marie Dangwang
    Monier, Guillaume
    Assadi, Aymen Amine
    Zeghioud, Hicham
    JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2022, 430
  • [3] Sulfur-doped g-C3N4/TiO2 S-scheme heterojunction photocatalyst for Congo Red photodegradation
    Wang, Juan
    Wang, Guohong
    Cheng, Bei
    Yu, Jiaguo
    Fan, Jiajie
    CHINESE JOURNAL OF CATALYSIS, 2021, 42 (01) : 56 - 68
  • [4] S-scheme g-C3N4/ZnO heterojunction photocatalyst with enhanced photodegradation of azo dye
    Lee, Ju-Ting
    Lee, Shu-Wen
    Wey, Ming-Yen
    JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS, 2022, 134
  • [5] Dual S-Scheme Heterojunction CdS/TiO2/g-C3N4 Photocatalyst for Hydrogen Production and Dye Degradation Applications
    Shoaib, Muhammad
    Naz, Muhammad Yasin
    Shukrullah, Shazia
    Munir, Muhammad Adnan
    Irfan, Muhammad
    Rahman, Saifur
    Ghanim, Abdulnoor Ali Jazem
    ACS OMEGA, 2023, 8 (45): : 43139 - 43150
  • [6] Understanding oxidation potential and degradation mechanism of acid-treated TiO2 coupled g-C3N4 S-scheme heterojunction photocatalyst for the removal of gaseous formaldehyde
    Maitlo, Hubdar Ali
    Younis, Sherif A.
    Kim, Ki-Hyun
    SEPARATION AND PURIFICATION TECHNOLOGY, 2025, 356
  • [7] A facile synthesis of SnS2/g-C3N4 S-scheme heterojunction photocatalyst with enhanced photocatalytic performance
    Thanh Huong Nguyen Thi
    Ha Tran Huu
    Hung Nguyen Phi
    Van Phuc Nguyen
    Quoc Dat Le
    Lan Nguyen Thi
    Thi Thuy Trang Phan
    Vien Vo
    JOURNAL OF SCIENCE-ADVANCED MATERIALS AND DEVICES, 2022, 7 (02):
  • [8] Fabrication of NiWO4/g-C3N4 S-scheme heterojunction photocatalyst for enhanced H2 evolution
    Wang, Wenqi
    Li, Chenxi
    Fan, Jun
    Sun, Tao
    Liu, Enzhou
    SURFACES AND INTERFACES, 2024, 44
  • [9] TiO2/BP/g-C3N4 heterojunction photocatalyst for the enhanced photocatalytic degradation of RhB
    Liu, Shujian
    Ge, Yanqing
    Wang, Chi
    Li, Kai
    Mei, Yi
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2023, 30 (35) : 84452 - 84461
  • [10] TiO2/BP/g-C3N4 heterojunction photocatalyst for the enhanced photocatalytic degradation of RhB
    Shujian Liu
    Yanqing Ge
    Chi Wang
    Kai Li
    Yi Mei
    Environmental Science and Pollution Research, 2023, 30 : 84452 - 84461