A novel phenol and ammonia recovery process for coal gasification wastewater altering the bacterial community and increasing pollutants removal in anaerobic/anoxic/aerobic system

被引:43
作者
Gui, Xuefei [1 ,2 ]
Xu, Weichao [1 ]
Cao, Hongbin [2 ,3 ]
Ning, Pengge [2 ]
Zhang, Yuxiu [1 ]
Li, Yuping [2 ]
Sheng, Yuxing [2 ,3 ]
机构
[1] China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China
[2] Chinese Acad Sci, CAS Interdisciplinary Innovat Team, Beijing 100190, Peoples R China
[3] Chinese Acad Sci, Inst Proc Engn, Natl Key Lab Biochem Engn, Beijing 100190, Peoples R China
基金
国家重点研发计划;
关键词
Coal gasification wastewater; Phenol and ammonia recovery; Biodegradability; Anaerobic/anoxic/aerobic system; Bacterial community; CONCEPTUAL DESIGN; BIODEGRADATION; DIGESTION; SLUDGE; PLANTS;
D O I
10.1016/j.scitotenv.2019.01.126
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Coal gasification wastewater (CGWW) is a typical toxic and refractory industrial wastewater. Here, a novel phenol and ammonia recovery process (IPE) was employed for CGWWpretreatment, and the coupled system assemble by the IPE process with A(2)/O system (IPE-A(2)/O) were operated to enhance the treatment performance of CGWW. The results showed that the IPE pre-treated effluent had a higher BOD5/COD ratio and lower refractory compounds compared to a typical process (MIBK). Subsequent A(2)/O biological treatment indicated that the A(2)/O-p system (A(2)/O system followed IPE process) obtained a higher average COD removal of 92% compared to 87.7% of the control (A(2)/O-m, A(2)/O system followed MIBK). The GC-MS analysis suggested that the content of alkanes in the IPE-A(2)/O effluent was lower than that of the MIBK-A(2)/O. The high-throughput sequencing revealed Levilinea, Alcaligenes, Acinetobacter, Thauera and Thiobacillus were the core genera in A(2)/O system. The genera Alcaligenes, Acinetobacter, Thauera and Thiobacillus in the degrading consortium were enriched in the A(2)/O-p system, leading to increased removals of organic pollutants and TN. These results suggested that the IPE process was a feasible pretreatment method, and the coupled IPE-A(2)/O system was an alternative technique for treating CGWW. (C) 2019 Published by Elsevier B.V.
引用
收藏
页码:203 / 211
页数:9
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