Selective Adsorption of Sulfur Dioxide in a Robust Metal-Organic Framework Material

被引：226

作者：

Savage, Mathew ^{[1
]}

Cheng, Yonggiong ^{[2
]}

Easun, Timothy L. ^{[3
]}

Eyley, Jennifer E. ^{[1
]}

Argent, Stephen P. ^{[4
]}

Warren, Mark R. ^{[5
]}

Lewis, William ^{[4
]}

Murray, Claire ^{[5
]}

Tang, Chiu C. ^{[5
]}

Frogley, Mark D. ^{[5
]}

Cinque, Gianfelice ^{[5
]}

Sun, Junliang ^{[6
]}

Rudic, Svemir ^{[7
]}

Murder, Richard T. ^{[8
]}

Benham, Michael J. ^{[8
]}

Fitch, Andrew N. ^{[9
]}

Blake, Alexander J. ^{[4
]}

Ramirez-Cuesta, Anibal J. ^{[2
]}

Yang, Sihai ^{[1
]}

Schroder, Martin ^{[1
]}

机构：

[1] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England

[2] Oak Ridge Natl Lab, CEMD, Neutron Sci Directorate, Oak Ridge, TN 37831 USA

[3] Cardiff Univ, Sch Chem, Cardiff CF10 3XQ, S Glam, Wales

[4] Univ Nottingham, Sch Chem, Univ Pk, Nottingham NG7 2RD, England

[5] Diamond Light Source, Harwell Sci Campus, Didcot OX11 ODE, Oxon, England

[6] Peking Univ, Coll Chem & Mol Engn, Beijing 100871, Peoples R China

[7] STFC Rutherford Appleton Lab, ISIS Neutron & Muon Source, Didcot OX11 0QX, Oxon, England

[8] Hiden Isochema, 422 Europa Blvd, Warrington WA5 7TS, Cheshire, England

[9] European Synchrotron Radiat Facil, F-38043 Grenoble, France

来源：

ADVANCED MATERIALS | 2016年 / 28卷 / 39期

基金：

英国工程与自然科学研究理事会;

关键词：

FLUE-GAS IMPURITIES; CARBON-DIOXIDE; CO2; ADSORPTION; POROUS HOST; STORAGE; HYDROCARBONS; CAPTURE; SEPARATIONS; POLLUTION; HYDROGEN;

D O I：

10.1002/adma.201602338

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Selective adsorption of SO2 is realized in a porous metal-organic framework material, and in-depth structural and spectroscopic investigations using Xrays, infrared, and neutrons define the underlying interactions that cause SO2 to bind more strongly than CO2 and N-2.

引用

页码：8705 / 8711

页数：7

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