Atmospheric mercury species measured in Guiyang, Guizhou province, southwest China

被引:43
|
作者
Liu, Na [1 ,2 ]
Qiu, Guangle [1 ]
Landis, Matthew S. [3 ]
Feng, Xinbin [1 ]
Fu, Xuewu [1 ]
Shang, Lihai [1 ]
机构
[1] Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550002, Peoples R China
[2] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
[3] US EPA, Off Resarch & Dev, Res Triangle Pk, NC 27709 USA
关键词
Atmospheric Hg; Speciation; Meteorological parameters; Anthropogenic sources; REACTIVE GASEOUS MERCURY; AMBIENT AIR; PARTICULATE MERCURY; ELEMENTAL MERCURY; DRY DEPOSITION; EASTERN SLOPE; EMISSIONS; URBAN; SOIL; SPECIATION;
D O I
10.1016/j.atmosres.2011.01.002
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Atmospheric mercury (Hg) species were measured in Guiyang City, the capital of Guizhou province, southwestern China at the Guiyang Monitoring Station Agency (GMSA) from September to November 2008 and at the Institute of Geochemistry, Chinese Academy of Sciences (IGCAS) during February, May, and July, 2009. Monitoring results found elevated concentrations of all three Hg species in ambient air in Guiyang. Large temporal and spatial variation patterns in the resulting data were also obtained. The overall average TGM concentrations at the GMSA and IGCAS sampling sites were 7.4 +/- 4.8 ng m(-3) and 6.2 +/- 5.1 ng m(-3), respectively. The average Hg(p) and RGM concentrations at GMSA were 1330 pg m(-3) and 24 pg m(-3), and at IGCAS were 250 pg m(-3) and 19 pg m(-3), respectively. It is hypothesized that local anthropogenic sources and the seasonal variability result in the high degree of spatial and temporal variability. (C) 2011 Elsevier B.V. All rights reserved.
引用
收藏
页码:93 / 102
页数:10
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