Highly Active and Stable Fe/SiO2 Catalyst Synthesized by Atomic Layer Deposition for CO Oxidation

被引:9
作者
Wang, Xiaofeng [1 ,4 ]
Jin, Baitang [1 ]
He, Xiaoqing [2 ]
White, Tommi A. [2 ,3 ]
Liang, Xinhua [1 ]
机构
[1] Missouri Univ Sci & Technol, Dept Chem & Biochem Engn, Rolla, MO 65409 USA
[2] Univ Missouri, Electron Microscopy Core Facil, Columbia, MO 65211 USA
[3] Univ Missouri, Dept Biochem, Columbia, MO 65211 USA
[4] Dalian Maritime Univ, Coll Environm Sci & Engn, Dalian 116026, Peoples R China
基金
美国国家科学基金会;
关键词
Iron nanoparticles; Atomic layer deposition; CO oxidation; SiO2; Stability; CARBON-MONOXIDE; IRON-OXIDES; NANOPARTICLES; TEMPERATURE; HYDROGENATION; NANOCATALYSTS; SHELL;
D O I
10.1007/s10562-020-03224-w
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Highly dispersed Fe nanoparticles (NPs) were deposited on SiO2 NPs by atomic layer deposition (ALD) in a scalable fluidized bed reactor at 400 oC. In CO oxidation reactions, over the Fe/SiO2 catalyst, Fe2O3 played a vital role. In a long-term stability test of more than 300 h of CO oxidation reaction, there was almost no activity decrease of Fe/SiO2 at 550 degrees C. [GRAPHICS] .
引用
收藏
页码:3296 / 3303
页数:8
相关论文
共 32 条
  • [1] Low-temperature CO oxidation over nanosized Fe-Co mixed oxide catalysts: Effect of calcination temperature and operational conditions
    Biabani-Ravandi, Abolfazl
    Rezaei, Mehran
    Fattah, Zohreh
    [J]. CHEMICAL ENGINEERING SCIENCE, 2013, 94 : 237 - 244
  • [2] Atomically dispersed iron hydroxide anchored on Pt for preferential oxidation of CO in H2
    Cao, Lina
    Liu, Wei
    Luo, Qiquan
    Yin, Ruoting
    Wang, Bing
    Weissenrieder, Jonas
    Soldemo, Markus
    Yan, Huan
    Lin, Yue
    Sun, Zhihu
    Ma, Chao
    Zhang, Wenhua
    Chen, Si
    Wang, Hengwei
    Guan, Qiaoqiao
    Yao, Tao
    Wei, Shiqiang
    Yang, Jinlong
    Lu, Junling
    [J]. NATURE, 2019, 565 (7741) : 631 - 635
  • [3] Synthesis of highly efficient α-Fe2O3 catalysts for CO oxidation derived from MIL-100(Fe)
    Cui, Lifeng
    Zhao, Di
    Yang, Yang
    Wang, Yuxin
    Zhang, Xiaodong
    [J]. JOURNAL OF SOLID STATE CHEMISTRY, 2017, 247 : 168 - 172
  • [4] deFaria DLA, 1997, J RAMAN SPECTROSC, V28, P873, DOI 10.1002/(SICI)1097-4555(199711)28:11<873::AID-JRS177>3.0.CO
  • [5] 2-B
  • [6] The influence of silver on the structural, redox and catalytic properties of the cryptomelane-type manganese oxides in the low-temperature CO oxidation reaction
    Gac, Wojciech
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2007, 75 (1-2) : 107 - 117
  • [7] Synthesis of supported Ni catalysts by atomic layer deposition
    Gould, Troy D.
    Lubers, Alia M.
    Neltner, Brian T.
    Carrier, Jacob V.
    Weimer, Alan W.
    Falconer, John L.
    Medlin, J. Will
    [J]. JOURNAL OF CATALYSIS, 2013, 303 : 9 - 15
  • [8] A Reactive Oxide Overlayer on Rhodium Nanoparticles during CO Oxidation and Its Size Dependence Studied by In Situ Ambient-Pressure X-ray Photoelectron Spectroscopy
    Grass, Michael E.
    Zhang, Yawen
    Butcher, Derek R.
    Park, Jeong Y.
    Li, Yimin
    Bluhm, Hendrik
    Bratlie, Kaitlin M.
    Zhang, Tianfu
    Somorjai, Gabor A.
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (46) : 8893 - 8896
  • [9] Chemoselective Transfer Hydrogenation of Nitroarenes Catalyzed by Highly Dispersed, Supported Nickel Nanoparticles
    Jiang, Chengjun
    Shang, Zeyu
    Liang, Xinhua
    [J]. ACS CATALYSIS, 2015, 5 (08): : 4814 - 4818
  • [10] Catalytic activity of Pt/SiO2 nanocatalysts synthesized via ultrasonic spray pyrolysis process under CO oxidation
    Jung, Chan-Ho
    Yun, Jaecheol
    Qadir, Kamran
    Naik, Brundabana
    Yun, Jung-Yeul
    Park, Jeong Young
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2014, 154 : 171 - 176