Rapid increase in dichloromethane emissions from China inferred through atmospheric observations

被引:52
作者
An, Minde [1 ,2 ]
Western, Luke M. [2 ]
Say, Daniel [2 ]
Chen, Liqu [3 ]
Claxton, Tom [4 ]
Ganesan, Anita L. [5 ]
Hossaini, Ryan [4 ,6 ]
Krummel, Paul B. [7 ]
Manning, Alistair J. [8 ]
Muhle, Jens [9 ]
O'Doherty, Simon [2 ]
Prinn, Ronald G. [10 ]
Weiss, Ray F. [9 ]
Young, Dickon [2 ]
Hu, Jianxin [1 ]
Yao, Bo [3 ,11 ,12 ]
Rigby, Matthew [2 ]
机构
[1] Peking Univ, Coll Environm Sci & Engn, Beijing, Peoples R China
[2] Univ Bristol, Sch Chem, Bristol, Avon, England
[3] China Meteorol Adm MOC CMA, Meteorol Observat Ctr, Beijing, Peoples R China
[4] Univ Lancaster, Lancaster Environm Ctr, Lancaster, England
[5] Univ Bristol, Sch Geog Sci, Bristol, Avon, England
[6] Univ Lancaster, Ctr Excellence Environm Data Sci, Lancaster, England
[7] CSIRO Oceans & Atmosphere, Climate Sci Ctr, Aspendale, Vic, Australia
[8] Hadley Ctr, Met Off, Exeter, Devon, England
[9] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA
[10] MIT, Ctr Global Change Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA
[11] Fudan Univ, Dept Atmospher & Ocean Sci, Shanghai, Peoples R China
[12] Fudan Univ, Inst Atmospher Sci, Shanghai, Peoples R China
基金
英国自然环境研究理事会; 美国海洋和大气管理局; 美国国家航空航天局; 欧盟地平线“2020”;
关键词
HALOGENATED COMPOUNDS; GLOBAL EMISSIONS; HFC EMISSIONS; IN-SITU; TRANSPORT; BROMINE; MODEL; HYDROCARBONS; HALOCARBONS; CHLOROFORM;
D O I
10.1038/s41467-021-27592-y
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Dichloromethane (CH2Cl2) is an unregulated ozone depleting substance whose emissions have strongly increased in recent years. Here, the authors show that rising emissions of dichloromethane in China between 2011 and 2019 can explain much of this global increase. With the successful implementation of the Montreal Protocol on Substances that Deplete the Ozone Layer, the atmospheric abundance of ozone-depleting substances continues to decrease slowly and the Antarctic ozone hole is showing signs of recovery. However, growing emissions of unregulated short-lived anthropogenic chlorocarbons are offsetting some of these gains. Here, we report an increase in emissions from China of the industrially produced chlorocarbon, dichloromethane (CH2Cl2). The emissions grew from 231 (213-245) Gg yr(-1) in 2011 to 628 (599-658) Gg yr(-1) in 2019, with an average annual increase of 13 (12-15) %, primarily from eastern China. The overall increase in CH2Cl2 emissions from China has the same magnitude as the global emission rise of 354 (281-427) Gg yr(-1) over the same period. If global CH2Cl2 emissions remain at 2019 levels, they could lead to a delay in Antarctic ozone recovery of around 5 years compared to a scenario with no CH2Cl2 emissions.
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页数:9
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