Thermal effects on arsenic emissions during coal combustion process

被引:20
|
作者
Zhang, Weiqiang [1 ,2 ]
Sun, Qiang [1 ,2 ,3 ]
Yang, Xiuyuan [4 ]
机构
[1] China Univ Min & Technol, Key Lab Coalbed Methane Resources & Reservoir For, Minist Educ, Xuzhou 221116, Jiangsu, Peoples R China
[2] China Univ Min & Technol, Sch Resources & Geosci, Xuzhou 221116, Jiangsu, Peoples R China
[3] Univ North Carolina Charlotte, Dept Civil & Environm Engn, Charlotte, NC 28223 USA
[4] China Geol Survey, Hydrogeol & Environm Geol Survey Ctr, Baoding 071051, Hebei, Peoples R China
关键词
Thermal effects; Emission rate; Arsenic; Coal combustion; Human health; TRACE-ELEMENTS; FLY-ASH; COCOMBUSTION; SPECIATION; FLUORINE;
D O I
10.1016/j.scitotenv.2017.08.262
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this study, the rate of emission of arsenic during the burning process of different kinds of coal is examined in order to study the volatile characteristics of arsenic during coal combustion which have negative effects on the ecological environment and human health. The results show that the emission rate of arsenic gradually increases with increased burning temperature, with a threshold of approximately 700 degrees C to 800 degrees C in the process of temperature increase. Then, the relationships among the arsenic emission rate and combustion environment, original arsenic content, combustion time, burning temperature, air flow and amount of arsenic fixing agent are discussed, and it is found that except for the original arsenic content, the rest of the factors have a nonlinear relationship with the emission rate of arsenic. That is, up to a certain level, they all contribute to the release of arsenic, and then their impact is minimal. The original arsenic content in coal is proportional to the arsenic emission rate. Therefore, taking into consideration the nonlinear relationships between factors that affect the arsenic emission rate can reduce contamination from arsenic. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:582 / 589
页数:8
相关论文
共 50 条
  • [21] Mechanism of arsenic migration and transformation during pulverized coal combustion
    Huang, Yongda
    Li, Aijun
    Hu, Hongyun
    Li, Shuai
    Zou, Chan
    Zou, Renjie
    Wu, Xiaojiang
    Naruse, Ichiro
    Yao, Hong
    PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2024, 40 (1-4)
  • [22] Regimes of association of arsenic and selenium during pulverized coal combustion
    Seames, Wayne S.
    Wendt, Jost O. L.
    PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2007, 31 : 2839 - 2846
  • [23] Volatilization of arsenic in coal during oxy-fuel combustion
    Department of Energy Power & Mechanical Engineering, North China Electric Power University, Baoding
    Hebei
    071003, China
    不详
    Hebei
    063009, China
    Huagong Xuebao, 12 (5079-5087):
  • [24] A dynamic model of the transformations of arsenic during coal combustion.
    Sterling, RO
    Helble, JJ
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2002, 224 : U582 - U582
  • [25] DISTRIBUTION OF ELEMENTS DURING THE PROCESS OF COAL COMBUSTION
    SODNOM, N
    GERBISH, S
    MASLOV, OD
    GAVRILOV, KA
    FIDERKEVICH, A
    ISOTOPENPRAXIS, 1989, 25 (07): : 286 - 289
  • [26] FUEL 125-Preliminary estimation of arsenic emissions from coal combustion in China
    Tian, Hezhong
    Qu, Yiping
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2008, 236
  • [27] Effect of Volatile and Ash Contents in Coal on the Volatilization of Arsenic during Isothermal Coal Combustion
    Zou, Chan
    Wang, Chunbo
    Liu, Huimin
    Wang, Hefei
    Zhang, Yue
    ENERGY & FUELS, 2017, 31 (11) : 12831 - 12838
  • [28] Migration and emissions of selenium during chemical looping combustion of coal
    Kang, Huifen
    Ma, Jingjing
    Guo, Xintong
    Han, Ziheng
    Hao, Jian
    Guo, Qingjie
    CANADIAN JOURNAL OF CHEMICAL ENGINEERING, 2023, 101 (05): : 2472 - 2484
  • [29] COAGGLOMERATION OF COAL AND LIMESTONE TO REDUCE SULFUR EMISSIONS DURING COMBUSTION
    MAJID, A
    SPARKS, BD
    CAPES, CE
    HAMER, CA
    FUEL, 1990, 69 (05) : 570 - 574
  • [30] Effects of limestone on polycyclic aromatic hydrocarbon emissions during coal atmospheric fluidized bed combustion
    Mastral, AM
    Garcia, T
    Callen, MS
    Lopez, JM
    Murillo, R
    Navarro, MV
    ENERGY & FUELS, 2001, 15 (06) : 1469 - 1474