High flux polyaniline-coated ceramic membrane for effective separation of emulsified oil-in-water

被引:19
作者
Salhi, Billel [1 ]
Baig, Nadeem [1 ]
Abdulazeez, Ismail [1 ]
Al-Ahmed, Amir [2 ]
Aljundi, Isam H. [1 ,3 ]
机构
[1] KFUPM, Interdisciplinary Res Ctr Membranes & Water Secur, Dhahran, Saudi Arabia
[2] KFUPM, Interdisciplinary Res Ctr Renewable Energy & Powe, Dhahran, Saudi Arabia
[3] King Fahd Univ Petr & Minerals, Chem Engn Dept, Dhahran 31261, Saudi Arabia
关键词
Demulsification; Ceramic membrane; Hybrid membranes; Polyaniline; Oil/water separation; MICROFILTRATION; NANOCOMPOSITES; SPECTRA;
D O I
10.1016/j.ceramint.2022.05.189
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Oil separation from oily wastewater is critical for environmental sustainability. In the present study, we report for the first time the facile fabrication of high flux polyaniline-modified ceramic membrane to effectively separate emulsified oil. Aniline was rapidly polymerized in a single step on alumina ceramic support using different monomer concentrations. It was revealed that the alumina membrane modified with 1.0 M aniline monomer is suitable for separating oil/water emulsions with an exceptionally high permeance of 3451 L m(-2).h(-1) (L.M.H.) and high separating efficiency. The polyaniline-coated alumina membranes appeared superhydrophilic/ superoleophobic w ith negligible fouling behavior. The modified membranes demonstrate a steady oil rejection flux after several cycles with excellent oil-rejection of 97%. The high flux, low operating pressure, and anti-fouling behavior revealed that these modified membranes are excellent candidates for emulsified-oil separation.
引用
收藏
页码:25246 / 25253
页数:8
相关论文
共 50 条
[31]   Heterogeneous wettability membrane for efficient demulsification and separation of oil-in-water emulsions [J].
Xu, Lang ;
Xu, Tianqi ;
Liu, Wenjing ;
Zuo, Tian ;
Wang, Teng ;
Cai, Ying ;
Zhang, Jiawen ;
Yi, Lingmin .
CHEMICAL ENGINEERING JOURNAL, 2024, 489
[32]   Preparation of corundum ceramic membrane with high permeability and corrosion resistance for oil in water separation [J].
Zhang, Enliang ;
Liu, Lulu ;
Jin, Shaowei ;
Zhao, Penghui ;
Wang, Xinzhen ;
Xu, Guogang .
CERAMICS INTERNATIONAL, 2025, 51 (12) :15512-15520
[33]   A novel ceramic microfiltration membrane fabricated by anthurium andraeanum-like attapulgite nanofibers for high-efficiency oil-in-water emulsions separation [J].
Fan, Zhaoru ;
Zhou, Shouyong ;
Mao, Hengyang ;
Li, Meisheng ;
Xue, Ailian ;
Zhao, Yijiang ;
Xing, Weihong .
JOURNAL OF MEMBRANE SCIENCE, 2021, 630
[34]   Fabrication of Attapulgite Coated Membranes for Effective Separation of Oil-in-Water Emulsion in Highly Acidic, Alkaline, and Concentrated Salty Environments [J].
Li, Jian ;
Zhao, Zhihong ;
Shen, Yongqian ;
Feng, Hua ;
Yang, Yaoxia ;
Zha, Fei .
ADVANCED MATERIALS INTERFACES, 2017, 4 (16)
[35]   Stability of oil-in-water emulsions produced by membrane emulsification with microporous ceramic membranes [J].
Zanatta, Vanessa ;
Rezzadori, Katia ;
Penha, Frederico Marques ;
Zin, Guilherme ;
Lemos-Senna, Elenara ;
Cunha Petrus, Jose Carlos ;
Di Luccio, Marco .
JOURNAL OF FOOD ENGINEERING, 2017, 195 :73-84
[36]   Polyaniline-Coated Electrospun Polyacrylonitrile Nanofibers for Effective Short-Chain PFAS (GenX) Removal from Water [J].
Jahan, Israt ;
Tani, Easmin Ara ;
Patel, Harsh V. ;
Zhao, Renzun ;
Zhang, Lifeng .
FIBERS, 2025, 13 (04)
[37]   Effective polysulfone-amorphous SiO2 NPs electrospun nanofiber membrane for high flux oil/water separation [J].
Obaid, M. ;
Tolba, Gehan M. K. ;
Motlak, Moaaed ;
Fadali, Olfat A. ;
Khalil, Abdelrazek Khalil ;
Almajid, Abdulhakim A. ;
Kim, Bongsoo ;
Barakat, Nasser A. M. .
CHEMICAL ENGINEERING JOURNAL, 2015, 279 :631-638
[38]   Lower-temperature preparation of SiC ceramic membrane using zeolite residue as sintering aid for oil-in-water separation [J].
Jiang, Qian ;
Zhou, Jian ;
Miao, Yu ;
Yang, Surui ;
Zhou, Ming ;
Zhong, Zhaoxiang ;
Xing, Weihong .
JOURNAL OF MEMBRANE SCIENCE, 2020, 610
[39]   A low-cost mullite-titania composite ceramic hollow fiber microfiltration membrane for highly efficient separation of oil-in-water emulsion [J].
Zhu, Li ;
Chen, Mingliang ;
Dong, Yingchao ;
Tang, Chuyang Y. ;
Huang, Aisheng ;
Li, Lingling .
WATER RESEARCH, 2016, 90 :277-285
[40]   Application of ceramic microfiltration membrane modified by nano-TiO2 coating in separation of a stable oil-in-water emulsion [J].
Chang, Qibing ;
Zhou, Jian-er ;
Wang, Yongqing ;
Liang, Jian ;
Zhang, Xiaozhen ;
Cerneaux, Sophie ;
Wang, Xia ;
Zhu, Zhiwen ;
Dong, Yingchao .
JOURNAL OF MEMBRANE SCIENCE, 2014, 456 :128-133