Stripper configurations for CO2 capture by aqueous monoethanolamine

被引:107
作者
Van Wagener, David H. [1 ]
Rochelle, Gary T. [1 ]
机构
[1] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA
关键词
Carbon dioxide; Monoethanolamine; Stripper; Reversibility; Efficiency;
D O I
10.1016/j.cherd.2010.11.011
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Absorption/stripping with amine solvents is a practical tail end technology for CO2 capture from coal-fired power plants. One of the inhibiting costs of this technology is the energy requirement for solvent regeneration in the stripper, but novel configurations can help reduce this requirement by making the process more reversible. This work looked at several configurations with varying levels of complexity to determine the most useful method for arranging process units. Evaluated configurations included multi-stage flash, multi-pressure columns, and advanced stripping columns. Using a higher number of pressure stages, packing in place of equilibrium flashes, and vapor recompression were all reasonable methods to reduce the overall equivalent work requirement, but the most significant improvement was seen with an interheated column. The interheated column and simple stripper required 33.4 kJ/mol CO2 and 35.0 kJ/mol CO2 of work, respectively, at their optimum lean loadings. 2010 The Institution of Chemical Engineers. Published by Elsevier B.V. Elsevier. All rights reserved.
引用
收藏
页码:1639 / 1646
页数:8
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