long-range transport;
PM10;
dust storm;
air pollutants;
impact;
D O I:
10.1016/j.atmosenv.2005.06.046
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
The impact of long-range transport on the air quality of Taiwan was assessed by using measurements at stations of the air quality monitoring network of the Taiwan Environment Protection Administration over the winter monsoon periods of 2000 and 2001. The primary long-range transport process can be clearly identified to be the prevailing northeasterly following the cold front of winter monsoon that originates in the Asian continent. Based on pollutants concentration differences among different meteorological conditions, we estimate that the long-range transport of particulate pollutants contributes to about 30 mu g m(-3) to the PM10 concentrations in northern and eastern Taiwan. A smaller contribution is estimated for the western plain of Taiwan. Contributions of the long-range transport to CO and SO2 are about 230 and 0.5 ppb, respectively. The identified, dust events have the highest average inflow concentration (about 71 +/- 34 mu g m(-3)) of PM10. The dust impacts on PM10 have been estimated to be nearly 100% at windward background stations along the north and northeast coast. In the northern cities of Taiwan, such as Taipei and Hsinchu, the impacts decrease to around 60-80% as local emission increase. Due to geographic blocking, a smaller impact is estimated for the western plain of Taiwan. However, the identified frontal pollution cases have significant impact on CO and SO2, which is more evident than the impact of dust events. In general, impacts of long-range transport on air pollutants at coastal stations are greater than those in urban areas. (c) 2005 Elsevier Ltd. All rights reserved.
机构:
CSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, IndiaCSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, India
Bikkina, Poonam
Sarma, V.V.S.S.
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机构:
CSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, IndiaCSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, India
Sarma, V.V.S.S.
Kawamura, Kimitaka
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机构:
Chubu University, Kasugai-shi,Aichi,487-8501, JapanCSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, India
Kawamura, Kimitaka
Bikkina, Srinivas
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机构:
Chubu University, Kasugai-shi,Aichi,487-8501, JapanCSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, India
Bikkina, Srinivas
Kunwar, Bhagawati
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机构:
Chubu University, Kasugai-shi,Aichi,487-8501, JapanCSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, India
Kunwar, Bhagawati
Sherin, C.K.
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机构:
Center for Marine Living Resources and Ecology, Kochi,Kerala,682508, IndiaCSIR-National Institute of Oceanography, Regional Centre, Visakhapatnam,Andhra Pradesh,530017, India
机构:
Drexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA
US EPA, Hosted, Washington, DC 20460 USADrexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA
Giordano, Michael R.
Kalnajs, Lars E.
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机构:
Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USADrexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA
Kalnajs, Lars E.
Avery, Anita
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Drexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USADrexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA
Avery, Anita
Goetz, J. Douglas
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Drexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USADrexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA
Goetz, J. Douglas
Davis, Sean M.
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机构:
NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO USA
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USADrexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA
Davis, Sean M.
DeCarlo, Peter F.
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机构:
Drexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA
Drexel Univ, Dept Chem, Philadelphia, PA 19104 USADrexel Univ, Dept Civil Architectural & Environm Engn, Philadelphia, PA 19104 USA