Ag2S/ZnO core-shell nanoheterojunction for a self-powered solid-state photodetector with wide spectral response

被引:26
作者
Chen, Duo [1 ,2 ]
Wei, Lin [3 ]
Wang, Dong [1 ,2 ]
Chen, Yanxue [1 ,2 ]
Tian, Yufeng [1 ,2 ]
Yan, Shishen [1 ,2 ]
Mei, Liangmo [1 ,2 ]
Jiao, Jun [4 ]
机构
[1] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China
[2] Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Shandong, Peoples R China
[3] Shandong Univ, Sch Microelect, Jinan 250100, Shandong, Peoples R China
[4] Portland State Univ, Dept Mech & Mat Engn, POB 751, Portland, OR 97207 USA
基金
中国国家自然科学基金;
关键词
Self-powered; Wide spectral response; Ag2S/ZnO core-shell; SOLAR-CELLS; ENHANCED PHOTORESPONSE;
D O I
10.1016/j.jallcom.2017.11.376
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
On the face of the impending energy crisis, developing low-energy consuming photoelectronic devices is extremely important. A wide spectral photosensitivity feature of a self-powered device provides an additional powerful tool. In this letter, a Ag2S/ZnO core-shell nanoheterojunction was prepared and a high performance self-powered solid-state photodetector was developed based on this nanostructure. High quality, vertically aligned ZnO nanoneedle arrays loaded with Ag2S quantum dotes were grown on FTO glass substrate by wet chemical methods. The microstructure and surface morphology of the prepared samples were characterized by transmission electron microscopy and scanning electron microscopy. A solid-state self-powered photodetector was assembled using this ZnO/Ag2S core-shell nanostructure as the photoanode. The photodetector shows a high photosensitivity in the wide spectral range from 400 to 1100 nm, and its response time is as short as 5 ms. Considering its excellent performance and easy fabrication process, this Ag2S/ZnO core-shell nanoheterojunction is an ideal candidate for wide spectral photodetecting application. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:2491 / 2496
页数:6
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