Optimal process design for the polygeneration of SNG, power and heat by hydrothermal gasification of waste biomass: Process optimisation for selected substrates

被引:32
作者
Gassner, Martin [1 ]
Vogel, Frederic [2 ]
Heyen, Georges [3 ]
Marechal, Francois [1 ]
机构
[1] Ecole Polytech Fed Lausanne, Ind Energy Syst Lab, CH-1015 Lausanne, Switzerland
[2] Paul Scherrer Inst, Lab Bioenergy & Catalysis, Villigen, Switzerland
[3] Univ Liege, Lab Anal & Synth Syst Chim, B-4000 Liege, Belgium
关键词
CONTINUOUS SALT PRECIPITATION; SYNTHETIC NATURAL-GAS; EQUATION-OF-STATE; CH4-CO2-H2O SYSTEM; 1000-DEGREES-C; SOLUBILITY; SEPARATION; MIXTURES; ENERGY; WATER;
D O I
10.1039/c0ee00634c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Based on a previously developed thermo-economic process model, this paper presents a detailed design study for the polygeneration of Synthetic Natural Gas (SNG), power and heat by catalytic hydrothermal gasification of biomass and biomass wastes in supercritical water. Using multi-objective optimisation techniques, the thermodynamic and thermo-economic performances of all candidate configurations from a general process superstructure are optimised with respect to SNG and electricity cogeneration and its associated investment cost, production cost and plant profitability. The paper demonstrates how both the optimal system configuration, its operating conditions and performances depend on the available technology, catalyst lifetime, process scale and the characteristics of the processed substrate.
引用
收藏
页码:1742 / 1758
页数:17
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