A versatile bio-based material for efficiently removing toxic dyes, heavy metal ions and emulsified oil droplets from water simultaneously

被引:55
作者
Li, Daikun [1 ]
Li, Qing [1 ]
Mao, Daoyong [1 ]
Bai, Ningning [1 ]
Dong, Hongzhou [1 ]
机构
[1] Southwest Univ, Sch Chem & Chem Engn, Tiansheng Rd 2, Chongqing 400715, Peoples R China
基金
中国国家自然科学基金;
关键词
Bio-based material; Toxic dyes; Heavy metal ions; Oil/water separation; OIL/WATER SEPARATION; AQUEOUS-SOLUTIONS; ADSORPTION-KINETICS; BETA-CYCLODEXTRIN; HYDROGEL BEADS; CATIONIC DYES; ANIONIC DYES; COATED MESH; ADSORBENT; MICROSPHERES;
D O I
10.1016/j.biortech.2017.09.016
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
Developing versatile materials for effective water purification is significant for environment and water source protection. Herein, a versatile bio-based material (CH-PAA-T) was reported by simple thermal cross-linking chitosan and polyacrylic acid which exhibits excellent performances for removing insoluble oil, soluble toxic dyes and heavy metal ions from water, simultaneously. The adsorption capacities are 990.1 mg g(-1) for methylene blue (MB) and 135.9 mg g(-1) for Cu2+, which are higher than most of present advanced absorbents. The adsorption towards organic dyes possesses high selectivity which makes CH-PAA-T be able to efficiently separate dye mixtures. The stable superoleophobicity under water endows CH-PAA-T good performance to separate toluene- in-water emulsion stabilized by Tween 80. Moreover, CH-PAA-T can be recycled for 10 times with negligible reduction of efficiency. Such versatile bio-based material is a potential candidate for water purification.
引用
收藏
页码:649 / 655
页数:7
相关论文
共 44 条
  • [1] A novel polyvinyltetrazole-grafted resin with high capacity for adsorption of Pb(II), Cu(II) and Cr(III) ions from aqueous solutions
    Chen, Youning
    He, Maofang
    Wang, Chaozhan
    Wei, Yinmao
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2014, 2 (27) : 10444 - 10453
  • [2] One-Step Fabrication of Graphene Oxide Enhanced Magnetic Composite Gel for Highly Efficient Dye Adsorption and Catalysis
    Cheng, Zehong
    Liao, Jie
    He, Benzhao
    Zhang, Fan
    Zhang, Faai
    Huang, Xiaohua
    Zhou, Li
    [J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2015, 3 (07): : 1677 - 1685
  • [3] Oil/Water Separation with Selective Superantiwetting/Superwetting Surface Materials
    Chu, Zonglin
    Feng, Yujun
    Seeger, Stefan
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2015, 54 (08) : 2328 - 2338
  • [4] Simple method for preparation of chitosan/poly(acrylic acid) blending hydrogel beads and adsorption of copper(II) from aqueous solutions
    Dai, Jie
    Yan, Han
    Yang, Hu
    Cheng, Rongshi
    [J]. CHEMICAL ENGINEERING JOURNAL, 2010, 165 (01) : 240 - 249
  • [5] Kinetic, equilibrium and thermodynamic phenomenological modeling of reactive dye adsorption onto polymeric adsorbent
    Dias Monte Blanco, Silvia Priscila
    Scheufele, Fabiano Bisinella
    Modenes, Aparecido Nivaldo
    Espinoza-Quinones, Fernando R.
    Marin, Pricila
    Kroumov, Alexander Dimitrov
    Borba, Carlos Eduardo
    [J]. CHEMICAL ENGINEERING JOURNAL, 2017, 307 : 466 - 475
  • [6] Multilayer Dye Adsorption in Activated Carbons-Facile Approach to Exploit Vacant Sites and Interlayer Charge Interaction
    Hadi, Pejman
    Guo, Jiaxin
    Barford, John
    McKay, Gordon
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2016, 50 (10) : 5041 - 5049
  • [7] Species differences in the metabolism of olefins: implications for risk assessment
    Henderson, RF
    [J]. CHEMICO-BIOLOGICAL INTERACTIONS, 2001, 135 : 53 - 64
  • [8] Mechanisms of lead adsorption on chitosan/PVA hydrogel beads
    Jin, L
    Bai, RB
    [J]. LANGMUIR, 2002, 18 (25) : 9765 - 9770
  • [9] Adsorption of anionic dyes on chitosan grafted poly(alkyl methacrylate)s
    Konaganti, Vinod Kumar
    Kota, Ramanjaneyulu
    Patil, Satish
    Madras, Giridhar
    [J]. CHEMICAL ENGINEERING JOURNAL, 2010, 158 (03) : 393 - 401
  • [10] Porous boron nitride nanosheets for effective water cleaning
    Lei, Weiwei
    Portehault, David
    Liu, Dan
    Qin, Si
    Chen, Ying
    [J]. NATURE COMMUNICATIONS, 2013, 4