Quench-resistant and stable nanocarbon dot/sheet emitters with tunable solid-state fluorescence via aggregation-induced color switching

被引:19
作者
Chang, Qing [1 ,2 ]
Ding, Yamei [1 ,2 ]
Cheng, Shuai [1 ,2 ]
Shen, Wei [3 ]
Zhou, Zhe [1 ,2 ]
Yin, Yuhang [1 ,2 ]
Sun, Tao [1 ,2 ]
Ban, Chaoyi [1 ,2 ]
Deng, Zhengtao [3 ]
Liu, Juqing [1 ,2 ]
Xiu, Fei [1 ,2 ]
Huang, Wei [1 ,2 ,4 ,5 ,6 ]
机构
[1] Nanjing Tech Univ NanjingTech, Key Lab Flexible Elect KLOFE, 30 South Puzhu Rd, Nanjing 211816, Jiangsu, Peoples R China
[2] Nanjing Tech Univ NanjingTech, IAM, 30 South Puzhu Rd, Nanjing 211816, Jiangsu, Peoples R China
[3] Nanjing Univ, Collaborat Innovat Ctr Chem Life Sci, Nanjing Natl Lab Microstruct, Dept Biomed Engn,Coll Engn & Appl Sci, 22 Hankou Rd, Nanjing 210093, Jiangsu, Peoples R China
[4] Nanjing Univ Posts & Telecommun, SICAM, Key Lab Organ Elect & Informat Displays, 9 Wenyuan Rd, Nanjing 210023, Jiangsu, Peoples R China
[5] Nanjing Univ Posts & Telecommun, SICAM, IAM, 9 Wenyuan Rd, Nanjing 210023, Jiangsu, Peoples R China
[6] NPU, SIFE, 127 West Youyi Rd, Xian 710072, Shaanxi, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
LIGHT-EMITTING-DIODES; CARBON DOTS; QUANTUM DOTS; EFFICIENT; EMISSION; NANODOTS; NANOTUBES; PHOSPHORS; GRAPHENE;
D O I
10.1039/c8nr08429g
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Nanocarbon fluorescence materials are promising color converters for multicolor emission via phosphor-coated light emitting devices (LEDs). Herein, a facile time-controlled solvothermal route was developed to prepare solid-state multicolor nanocarbon emitters comprising dot/sheet nanohybrids. The nanocarbons demonstrate an aggregation-induced color switching behavior, leading to tunable light emission from blue to yellow by modulating the solvothermal reaction time. Particularly, these emitters show outstanding film-forming ability directly and a high production yield (approximate to 40%). Moreover, the nanocarbon-coated ultraviolet LEDs exhibit high quality multicolor light emission and excellent color stability at high voltages, impelling the development of emerging carbon phosphors in fundamental research studies and practical applications.
引用
收藏
页码:2131 / 2137
页数:7
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