Per- and polyfluoroalkyl substances in the environment

被引：958

作者：

Evich, Marina G. ^{[1
]}

Davis, Mary J. B. ^{[1
]}

McCord, James P. ^{[2
]}

Acrey, Brad ^{[1
]}

Awkerman, Jill A. ^{[3
]}

Knappe, Detlef R. U. ^{[4
,5
]}

Lindstrom, Andrew B. ^{[6
]}

Speth, Thomas F. ^{[7
]}

Tebes-Stevens, Caroline ^{[1
]}

Strynar, Mark J. ^{[2
]}

Wang, Zhanyun ^{[8
]}

Weber, Eric J. ^{[1
]}

Henderson, W. Matthew ^{[1
]}

Washington, John W. ^{[1
,9
]}

机构：

[1] US EPA, Off Res & Dev ORD, Ctr Environm Measurement & Modeling, Athens, GA 30605 USA

[2] US EPA, ORD, Ctr Environm Measurement & Modeling, Durham, NC 27711 USA

[3] US EPA, ORD, Ctr Environm Measurement & Modeling, Gulf Breeze, FL 32561 USA

[4] North Carolina State Univ, Dept Civil Construct & Environm Engneerirg, Raleigh, NC 27695 USA

[5] North Carolina State Univ, Ctr Human Hlth & Environm, Raleigh, NC 27695 USA

[6] US EPA, ORD, Ctr Publ Hlth & Environm Assessment, Durham, NC 27711 USA

[7] US EPA, ORD, Ctr Environm Solut & Emergency Response, Cincinnati, OH 45268 USA

[8] Swiss Fed Inst Technol, Inst Environm Engn, CH-8093 Zurich, Switzerland

[9] Univ Georgia, Dept Geol, Athens, GA 30602 USA

来源：

SCIENCE | 2022年 / 375卷 / 6580期

基金：

美国国家卫生研究院;

关键词：

8/2 FLUOROTELOMER ALCOHOL; PERFLUORINATED CARBOXYLIC-ACIDS; GLOBAL EMISSION INVENTORIES; FILM-FORMING FOAM; PERFLUOROALKYL SUBSTANCES; AEROBIC BIOTRANSFORMATION; POLYFLUORINATED COMPOUNDS; PERFLUOROOCTANE SULFONATE; TROPHIC MAGNIFICATION; PFCA HOMOLOGS;

D O I：

10.1126/science.abg9065

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

Over the past several years, the term PFAS (per- and polyfluoroalkyl substances) has grown to be emblematic of environmental contamination, garnering public, scientific, and regulatory concern. PFAS are synthesized by two processes, direct fluorination (e.g., electrochemical fluorination) and oligomerization (e.g., fluorotelomerization). More than a megatonne of PFAS is produced yearly, and thousands of PFAS wind up in end-use products. Atmospheric and aqueous fugitive releases during manufacturing, use, and disposal have resulted in the global distribution of these compounds. Volatile PFAS facilitate long-range transport, commonly followed by complex transformation schemes to recalcitrant terminal PFAS, which do not degrade under environmental conditions and thus migrate through the environment and accumulate in biota through multiple pathways. Efforts to remediate PFAS-contaminated matrices still are in their infancy, with much current research targeting drinking water.

引用

页码：512 / +

页数：15

共 163 条

[11] First assessment on degradability of sodium p-perfluorous nonenoxybenzene sulfonate (OBS), a high volume alternative to perfluorooctane sulfonate in fire-fighting foams and oil production agents in China [J].

Bao, Yixiang ;

Qu, Yingxi ;

Huang, Jun ;

Cagnetta, Giovanni ;

Yu, Gang ;

Weber, Roland .

RSC ADVANCES, 2017, 7 (74) :46948-46957

[12] Critical review on PFOA, kidney cancer, and testicular cancer [J].

Bartell, Scott M. ;

Vieira, Veronica M. .

JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2021, 71 (06) :663-679

[13] Investigation of an immobilization process for PFAS contaminated soils* [J].

Barth, Edwin ;

McKernan, John ;

Bless, Diana ;

Dasu, Kavitha .

JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2021, 296

[14] Discovery of 40 Classes of Per- and Polyfluoroalkyl Substances in Historical Aqueous Film-Forming Foams (AFFFs) and AFFF-Impacted Groundwater [J].

Barzen-Hanson, Krista A. ;

Roberts, Simon C. ;

Choyke, Sarah ;

Oetjen, Karl ;

McAlees, Alan ;

Riddell, Nicole ;

McCrindle, Robert ;

Ferguson, P. Lee ;

Higgins, Christopher P. ;

Field, Jennifer A. .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2017, 51 (04) :2047-2057

[15] A forensic approach for distinguishing PFAS materials [J].

Benotti, Mark J. ;

Fernandez, Loretta A. ;

Peaslee, Graham F. ;

Douglas, Gregory S. ;

Uhler, Allen D. ;

Emsbo-Mattingly, Stephen .

ENVIRONMENTAL FORENSICS, 2020, 21 (3-4) :319-333

[16] Biodegradation of N-Ethyl Perfluorooctane Sulfonamido Ethanol (EtFOSE) and EtFOSE-Based Phosphate Diester (SAmPAP Diester) in Marine Sediments [J].

Benskin, Jonathan P. ;

Ikonomou, Michael G. ;

Gobas, Frank A. P. C. ;

Begley, Timothy H. ;

Woudneh, Million B. ;

Cosgrove, John R. .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2013, 47 (03) :1381-1389

[17] Uptake of perfluorooctanoic acid, perfluorooctane sulfonate and perfluorooctane sulfonamide by carrot and lettuce from compost amended soil [J].

Bizkarguenaga, E. ;

Zabaleta, I. ;

Mijangos, L. ;

Iparraguirre, A. ;

Fernandez, L. A. ;

Prieto, A. ;

Zuloaga, O. .

SCIENCE OF THE TOTAL ENVIRONMENT, 2016, 571 :444-451

[18] Perfluoroalkyl Acid Uptake in Lettuce (Lactuca sativa) and Strawberry (Fragaria ananassa) Irrigated with Reclaimed Water [J].

Blaine, Andrea C. ;

Rich, Courtney D. ;

Sedlacko, Erin M. ;

Hyland, Katherine C. ;

Stushnoff, Cecil ;

Dickenson, Eric R. V. ;

Higgins, Christopher P. .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (24) :14361-14368

[19] Perfluoroalkyl Acid Distribution in Various Plant Compartments of Edible Crops Grown in Biosolids-Amended soils [J].

Blaine, Andrea C. ;

Rich, Courtney D. ;

Sedlacko, Erin M. ;

Hundal, Lakhwinder S. ;

Kumar, Kuldip ;

Lau, Christopher ;

Mills, Marc A. ;

Harris, Kimberly M. ;

Higgins, Christopher P. .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (14) :7858-7865

[20] Uptake of Perfluoroalkyl Acids into Edible Crops via Land Applied Biosolids: Field and Greenhouse Studies [J].

Blaine, Andrea C. ;

Rich, Courtney D. ;

Hundal, Lakhwinder S. ;

Lau, Christopher ;

Mills, Marc A. ;

Harris, Kimberly M. ;

Higgins, Christopher P. .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2013, 47 (24) :14062-14069

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