Unveiling the influential mechanism of O2 on the corrosion of N80 carbon steel under dynamic supercritical CO2 conditions

被引：7

作者：

Li, Y. Y. ^{[1
]}

Jiang, Z. N. ^{[1
]}

Zhang, Q. H. ^{[1
]}

Lei, Y. ^{[1
]}

Wang, X. ^{[1
]}

Zhang, G. A. ^{[1
]}

机构：

[1] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Hubei Key Lab Mat Chem & Serv Failure, Key Lab Mat Chem Energy Convers & Storage,Minist, Wuhan 430074, Peoples R China

来源：

CORROSION SCIENCE | 2022年 / 205卷

基金：

中国国家自然科学基金;

关键词：

Supercritical CO2-O-2; Waterchemistrymodel; Steelcorrosion; Electrochemicalmeasurements; Diffusionbarriereffect; LOW-TEMPERATURE OXIDATION; PRESSURE AIR INJECTION; GEOLOGICAL SEQUESTRATION; MUTUAL SOLUBILITIES; CO2-H2O MIXTURES; AQUEOUS NACL; STORAGE CCS; WATER; BEHAVIOR; CAPTURE;

D O I：

10.1016/j.corsci.2022.110436

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

The influential mechanism of O-2 on the corrosion of N80 carbon steel under dynamic supercritical CO2 conditions was explored by mass loss and electrochemical tests, and surface analysis. It is demonstrated that the introduction of O-2 inhibits the corrosion of steel. The developed water chemistry model confirms that the decrease in the corrosive species concentration by introducing O-2 is not responsible for the inhibition to steel corrosion. The corrosion inhibition of O-2 is implemented by promoting the formation of protective FeCO3 film in the initial period owing to the diffusion barrier effect of the formed outer ferric hydroxide/oxide film.

引用

页数：20

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