Light amplification in semiconductor nanocrystals: Quantum rods versus quantum dots

被引:143
作者
Htoon, H [1 ]
Hollingworth, JA [1 ]
Malko, AV [1 ]
Dickerson, R [1 ]
Klimov, VI [1 ]
机构
[1] Los Alamos Natl Lab, Los Alamos, NM 87545 USA
关键词
D O I
10.1063/1.1586460
中图分类号
O59 [应用物理学];
学科分类号
摘要
We perform side-by-side comparison of optical gain properties of spherical and elongated nanocrystals (quantum dots and quantum rods, respectively). This comparison indicates that elongated nanoparticles provide several features beneficial for lasing applications, such as enhanced absorption cross sections (and hence reduced lasing threshold and improved photostability), increased optical gain lifetime, and extended optical gain spectral range through the use of transitions that involve both ground and excited electronic states. (C) 2003 American Institute of Physics.
引用
收藏
页码:4776 / 4778
页数:3
相关论文
共 15 条
[1]   Semiconductor nanocrystals as fluorescent biological labels [J].
Bruchez, M ;
Moronne, M ;
Gin, P ;
Weiss, S ;
Alivisatos, AP .
SCIENCE, 1998, 281 (5385) :2013-2016
[2]   Electroluminescence from single monolayers of nanocrystals in molecular organic devices [J].
Coe, S ;
Woo, WK ;
Bawendi, M ;
Bulovic, V .
NATURE, 2002, 420 (6917) :800-803
[3]   Color-selective semiconductor nanocrystal laser [J].
Eisler, HJ ;
Sundar, VC ;
Bawendi, MG ;
Walsh, M ;
Smith, HI ;
Klimov, V .
APPLIED PHYSICS LETTERS, 2002, 80 (24) :4614-4616
[4]   Size-dependent tunneling and optical spectroscopy of CdSe quantum rods [J].
Katz, D ;
Wizansky, T ;
Millo, O ;
Rothenberg, E ;
Mokari, T ;
Banin, U .
PHYSICAL REVIEW LETTERS, 2002, 89 (08)
[5]  
Kazes M, 2002, ADV MATER, V14, P317, DOI 10.1002/1521-4095(20020219)14:4<317::AID-ADMA317>3.3.CO
[6]  
2-L
[7]   Optical gain and stimulated emission in nanocrystal quantum dots [J].
Klimov, VI ;
Mikhailovsky, AA ;
Xu, S ;
Malko, A ;
Hollingsworth, JA ;
Leatherdale, CA ;
Eisler, HJ ;
Bawendi, MG .
SCIENCE, 2000, 290 (5490) :314-317
[8]   Quantization of multiparticle Auger rates in semiconductor quantum dots [J].
Klimov, VI ;
Mikhailovsky, AA ;
McBranch, DW ;
Leatherdale, CA ;
Bawendi, MG .
SCIENCE, 2000, 287 (5455) :1011-1013
[9]   Ultrafast carrier dynamics, optical amplification, and lasing in nanocrystal quantum dots [J].
Klimov, VI ;
Bawendi, MG .
MRS BULLETIN, 2001, 26 (12) :998-1004
[10]   Optical nonlinearities and ultrafast carrier dynamics in semiconductor nanocrystals [J].
Klimov, VI .
JOURNAL OF PHYSICAL CHEMISTRY B, 2000, 104 (26) :6112-6123