Oil-mineral aggregate formation on oiled beaches:: Natural attenuation and sediment relocation

被引:59
作者
Lee, K
Stoffyn-Egli, P
Tremblay, GH
Owens, EH
Sergy, GA
Guénette, CC
Prince, RC
机构
[1] Fisheries & Oceans Canada, Bedford Inst Oceanog, Ctr Offshore Oil & Gas Environm Res, Dartmouth, NS B2Y 4A2, Canada
[2] BDR Res Ltd, Halifax, NS B3J 2T3, Canada
[3] Polaris Appl Sci Inc, Bainbridge Isl, WA 98110 USA
[4] Environm Canada, Edmonton, AB T6B 2X3, Canada
[5] SINTEF Appl Chem, Environm Engn, N-7034 Trondheim, Norway
[6] ExxonMobil Res & Engn Co, Annandale, NJ 08801 USA
[7] Fisheries & Oceans Canada, Maurice Lamontagne Inst, Reg Oceans & Environm Branch, Mont Joli, PQ GSH 324, Canada
关键词
oil spill remediation; oil dispersion; oil-mineral aggregation; fine sediment; biodegradation;
D O I
10.1016/S1353-2561(03)00042-2
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The significance of oil-mineral aggregate (OMA) formation on the effectiveness of the in situ shoreline treatment options of natural attenuation (natural recovery) and sediment relocation (surf washing) was examined during field trials on two mixed-sediment (sand and pebble) beaches experimentally oiled with IF-30 oil. At both sites, the amount of oil remaining in the experimental plots was dramatically reduced within five days after sediment relocation treatments. Time-series microscopy and image analysis of breaker-zone water samples demonstrate that OMA formation occurred naturally on the oiled beaches at both sites and was accelerated by the sediment relocation procedure. Lower concentrations of OMA in the breaker zone at Site 3 are attributed to the higher wave-energy levels at this site that presumably facilitated more rapid OMA dispersion. The granulometry and mineralogy of beach sediment and of subtidal sediment trap samples indicate that the material settling in nearshore waters originated from the relocated sediment and that a portion of the finer sediment was probably transported out of the study region before settling. Gas chromatography/mass spectrometry analysis demonstrated that a significant fraction of the oil dispersed into nearshore waters and sediments by interaction with mineral fines was biodegraded. The fact that little or no residual oil was found stranded on the shore in areas adjacent to the experimental plots and that only small amounts of oil were found in nearshore subtidal sediments and sediment trap samples suggests that a large fraction of the oil lost from the experimental plots may have been dispersed in the form of relatively buoyant OMA. Crown Copyright (C) 2003 Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:285 / 296
页数:12
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