Improve the slurry ability of lignite through co-slurrying and microwave co-pyrolysis with direct coal liquefaction residue

被引:7
作者
Ren, Yangguang [1 ]
Gu, Suqian [2 ,3 ]
Xu, Zhiqiang [2 ]
Wang, Qun [1 ]
机构
[1] Shandong Univ Sci & Technol, Sch Chem & Biol Engn, Qingdao 266590, Peoples R China
[2] China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China
[3] China Univ Min & Technol Beijing, D11 Xueyuan Rd, Beijing 100083, Peoples R China
基金
中国国家自然科学基金;
关键词
Lignite; Direct coal liquefaction residue; Co-slurry; Microwave co-pyrolysis; Upgraded lignite water slurry; LOW-TEMPERATURE PYROLYSIS; LOW-RANK COAL; ASSISTED PYROLYSIS; INDONESIAN LIGNITE; PETROLEUM COKE; PORE STRUCTURE; SLURRYABILITY; IRRADIATION; PERFORMANCE; FACILITATE;
D O I
10.1016/j.jaap.2022.105559
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
This study is devoted to demonstrating experimentally the advantages of direct coal liquefaction residue (DCLR) on improving the slurry ability of lignite through co-slurry and microwave co-pyrolysis. The results show that: as the lignite/DCLR mass ratio decreased from 10:0-5:5 the maximum solid concentration (MSC) of the mixed slurry increased from 42.14 wt% to 54.25 wt%, simultaneously, the pseudoplasticity and static stability gradually decreased. This is because the organic matter and abundant minerals in DCLR remarkably changed the slurry ability of mixed slurry. And during microwave pyrolysis with the assist of 12 wt% DCLR the slow drying stage of lignite pyrolysis was shortened, and the constant temperature stage was extended, thus, the coal quality was improved, the oxygen-containing functional groups was removed significantly and the BET specific surface area increased. These changes caused the MSC of upgraded lignite water slurry (ULWS) increased to 64.54 wt%; but the "shear-thinning" characteristic became inconspicuous, and the static stability became slightly worse. In general, DCLR could effectively improve the slurry ability of lignite through co-slurry with lignite at a mass ratio of 5:5 and co-pyrolysis with lignite at a microwave power of 1000 W.
引用
收藏
页数:12
相关论文
共 49 条
[1]   Microwave-assisted pyrolysis of Mississippi coal: A comparative study with conventional pyrolysis [J].
Abdelsayed, Victor ;
Shekhawat, Dushyant ;
Smith, Mark W. ;
Link, Dirk ;
Stiegman, Albert E. .
FUEL, 2018, 217 :656-667
[2]   Direct liquefaction techniques on lignite coal: A review [J].
Ali, Arif ;
Zhao, Chen .
CHINESE JOURNAL OF CATALYSIS, 2020, 41 (03) :375-389
[3]   Mechanism of synergy effect during microwave co-pyrolysis of biomass and lignite [J].
An, Yang ;
Tahmasebi, Arash ;
Yu, Jianglong .
JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS, 2017, 128 :75-82
[4]   Thermal behaviour during the pyrolysis of low rank perhydrous coals [J].
Arenillas, A ;
Rubiera, F ;
Pis, JJ ;
Cuesta, MJ ;
Iglesias, MJ ;
Jiménez, A ;
Suárez-Ruis, I .
JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS, 2003, 68-9 :371-385
[5]   Preparation of high concentration coal water slurry of lignite based on surface modification using the second fluid and the second particle [J].
Chen, Xing ;
Wang, Chunyu ;
Wang, Ziyu ;
Zhao, Hui ;
Liu, Haifeng .
FUEL, 2019, 242 :788-793
[6]   Predicting the degree of surface oxidation on fine coals by measuring the oxygen transfer rate in coal suspensions [J].
Chen, Xumeng ;
Chang, Ziyong ;
Peng, Yongjun .
FUEL PROCESSING TECHNOLOGY, 2017, 159 :313-319
[7]   Physicochemical characterizations for improving the slurryability of Philippine lignite upgraded through microwave irradiation [J].
Cheng, Jun ;
Wang, Xin ;
Zhou, Fan ;
Huang, Rui ;
Wang, Aiying ;
Chen, Xungang ;
Liu, Jianzhong ;
Cen, Kefa .
RSC ADVANCES, 2015, 5 (19) :14690-14696
[8]   Combined effects of additives and power levels on microwave drying performance of lignite thin layer [J].
Fu, B. A. ;
Chen, M. Q. ;
Huang, Y. W. ;
Luo, H. F. .
DRYING TECHNOLOGY, 2017, 35 (02) :227-239
[9]   Extraction and sequential elution of a heavy oil from direct coal liquefaction [J].
Gao, Hua-Shuai ;
Zong, Zhi-Min ;
Yang, Zheng ;
Huang, Li-Li ;
Zhang, Min ;
Teng, Dao-Guang ;
Wei, Xian-Yong .
FUEL, 2020, 260
[10]   Dynamic migration mechanism of organic oxygen in Fugu coal pyrolysis by large-scale ReaxFF molecular dynamics [J].
Gao, Mingjie ;
Li, Xiaoxia ;
Guo, Xin ;
Chen, Lei ;
Sun, Laizhi ;
Yang, Shuangxia ;
Xie, Xinping ;
Hua, Dongliang .
JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS, 2021, 156