AirCore: An Innovative Atmospheric Sampling System

被引:156
作者
Karion, Anna [1 ,2 ]
Sweeney, Colm [1 ,2 ]
Tans, Pieter [1 ]
Newberger, Timothy [3 ]
机构
[1] NOAA, ESRL, Boulder, CO 80305 USA
[2] Univ Colorado, CIRES, Boulder, CO 80309 USA
[3] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY USA
关键词
IN-SITU OBSERVATIONS; CARBON-DIOXIDE; CO2; AIRCRAFT; CH4; AIR; ANALYZER; SURFACE; SINKS; FLUX;
D O I
10.1175/2010JTECHA1448.1
中图分类号
P75 [海洋工程];
学科分类号
0814 ; 081505 ; 0824 ; 082401 ;
摘要
This work describes the Air Core, a simple and innovative atmospheric sampling system. The AirCore used in this study is a 150-m-long stainless steel tube, open at one end and closed at the other, that relies on positive changes in ambient pressure for passive sampling of the atmosphere. The Air Core evacuates while ascending to a high altitude and collects a sample of the ambient air as it descends. It is sealed upon recovery and measured with a continuous analyzer for trace gas mole fraction. The Air Core tubing can be shaped into a variety of configurations to accommodate any sampling platform; for the testing done in this work it was shaped into a 0,75-m-diameter coil. Measurements of CO2 and CH4 mole fractions in laboratory tests indicate a repeatability and lack of bias to better than 0.07 ppm (one sigma) for CO, and 0.4 ppb for CH4 under various conditions. Comparisons of AirCore data with flask data from aircraft flights indicate a standard deviation of differences of 0.3 ppm and 5 ppb for CO2 and CH4, respectively, with no apparent bias. Accounting for longitudinal mixing, the expected measurement resolution for CO2 is 110 m at sea level, 260 m at 8000 m. and 1500 m at 20 000 m ASL after 3 h of storage, decreasing to 170, 390, and 2300 m, after 12 h. Validation tests confirm that the AirCore is a robust sampling device for many species on a variety of platforms, including balloons, unmanned aerial vehicles (UAVs), and aircraft.
引用
收藏
页码:1839 / 1853
页数:15
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