AirCore: An Innovative Atmospheric Sampling System

被引:156
作者
Karion, Anna [1 ,2 ]
Sweeney, Colm [1 ,2 ]
Tans, Pieter [1 ]
Newberger, Timothy [3 ]
机构
[1] NOAA, ESRL, Boulder, CO 80305 USA
[2] Univ Colorado, CIRES, Boulder, CO 80309 USA
[3] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY USA
关键词
IN-SITU OBSERVATIONS; CARBON-DIOXIDE; CO2; AIRCRAFT; CH4; AIR; ANALYZER; SURFACE; SINKS; FLUX;
D O I
10.1175/2010JTECHA1448.1
中图分类号
P75 [海洋工程];
学科分类号
0814 ; 081505 ; 0824 ; 082401 ;
摘要
This work describes the Air Core, a simple and innovative atmospheric sampling system. The AirCore used in this study is a 150-m-long stainless steel tube, open at one end and closed at the other, that relies on positive changes in ambient pressure for passive sampling of the atmosphere. The Air Core evacuates while ascending to a high altitude and collects a sample of the ambient air as it descends. It is sealed upon recovery and measured with a continuous analyzer for trace gas mole fraction. The Air Core tubing can be shaped into a variety of configurations to accommodate any sampling platform; for the testing done in this work it was shaped into a 0,75-m-diameter coil. Measurements of CO2 and CH4 mole fractions in laboratory tests indicate a repeatability and lack of bias to better than 0.07 ppm (one sigma) for CO, and 0.4 ppb for CH4 under various conditions. Comparisons of AirCore data with flask data from aircraft flights indicate a standard deviation of differences of 0.3 ppm and 5 ppb for CO2 and CH4, respectively, with no apparent bias. Accounting for longitudinal mixing, the expected measurement resolution for CO2 is 110 m at sea level, 260 m at 8000 m. and 1500 m at 20 000 m ASL after 3 h of storage, decreasing to 170, 390, and 2300 m, after 12 h. Validation tests confirm that the AirCore is a robust sampling device for many species on a variety of platforms, including balloons, unmanned aerial vehicles (UAVs), and aircraft.
引用
收藏
页码:1839 / 1853
页数:15
相关论文
共 34 条
[1]   Empirical age spectra for the lower tropical stratosphere from in situ observations of CO2:: Implications for stratospheric transport [J].
Andrews, AE ;
Boering, KA ;
Daube, BC ;
Wofsy, SC ;
Hintsa, EJ ;
Weinstock, EM ;
Bui, TP .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D21) :26581-26595
[2]   Mean ages of stratospheric air derived from in situ observations of CO2, CH4, and N2O [J].
Andrews, AE ;
Boering, KA ;
Daube, BC ;
Wofsy, SC ;
Loewenstein, M ;
Jost, H ;
Podolske, JR ;
Webster, CR ;
Herman, RL ;
Scott, DC ;
Flesch, GJ ;
Moyer, EJ ;
Elkins, JW ;
Dutton, GS ;
Hurst, DF ;
Moore, FL ;
Ray, EA ;
Romashkin, PA ;
Strahan, SE .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D23) :32295-32314
[3]   ON THE DISPERSION OF A SOLUTE IN A FLUID FLOWING THROUGH A TUBE [J].
ARIS, R .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1956, 235 (1200) :67-77
[4]   TransCom 3 inversion intercomparison:: Impact of transport model errors on the interannual variability of regional CO2 fluxes, 1988-2003 -: art. no. GB1002 [J].
Baker, DF ;
Law, RM ;
Gurney, KR ;
Rayner, P ;
Peylin, P ;
Denning, AS ;
Bousquet, P ;
Bruhwiler, L ;
Chen, YH ;
Ciais, P ;
Fung, IY ;
Heimann, M ;
John, J ;
Maki, T ;
Maksyutov, S ;
Masarie, K ;
Prather, M ;
Pak, B ;
Taguchi, S ;
Zhu, Z .
GLOBAL BIOGEOCHEMICAL CYCLES, 2006, 20 (01)
[5]   Strategies for measurement of atmospheric column means of carbon dioxide from aircraft using discrete sampling [J].
Bakwin, PS ;
Tans, PP ;
Stephens, BB ;
Wofsy, SC ;
Gerbig, C ;
Grainger, A .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D16)
[6]   High-accuracy continuous airborne measurements of greenhouse gases (CO2 and CH4) using the cavity ring-down spectroscopy (CRDS) technique [J].
Chen, H. ;
Winderlich, J. ;
Gerbig, C. ;
Hoefer, A. ;
Rella, C. W. ;
Crosson, E. R. ;
Van Pelt, A. D. ;
Steinbach, J. ;
Kolle, O. ;
Beck, V. ;
Daube, B. C. ;
Gottlieb, E. W. ;
Chow, V. Y. ;
Santoni, G. W. ;
Wofsy, S. C. .
ATMOSPHERIC MEASUREMENT TECHNIQUES, 2010, 3 (02) :375-386
[7]   Net fluxes of CO2 in Amazonia derived from aircraft observations -: art. no. 4614 [J].
Chou, WW ;
Wofsy, SC ;
Harriss, RC ;
Lin, JC ;
Gerbig, C ;
Sachse, GW .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D22)
[8]   EVIDENCE FOR INTERANNUAL VARIABILITY OF THE CARBON-CYCLE FROM THE NATIONAL-OCEANIC-AND-ATMOSPHERIC-ADMINISTRATION CLIMATE-MONITORING-AND-DIAGNOSTICS-LABORATORY GLOBAL-AIR-SAMPLING-NETWORK [J].
CONWAY, TJ ;
TANS, PP ;
WATERMAN, LS ;
THONING, KW .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1994, 99 (D11) :22831-22855
[9]  
CREVOISIER C, 2010, P NATL ACAD IN PRESS
[10]   A direct carbon budgeting approach to infer carbon sources and sinks. Design and synthetic application to complement the NACP observation network [J].
Crevoisier, Cyril ;
Gloor, Manuel ;
Gloaguen, Erwan ;
Horowitz, Larry W. ;
Sarmiento, Jorge L. ;
Sweeney, Colm ;
Tans, Pieter P. .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2006, 58 (05) :366-375