Decoherence of molecular vibrational wave packets: Observable manifestations and control criteria

被引：41
作者：
Brif, C [1 ]
Rabitz, H
Wallentowitz, S
Walmsley, IA
机构：
[1] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
[2] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA
[3] Univ Rochester, Rochester Theory Ctr Opt Sci & Engn, Rochester, NY 14627 USA
[4] Univ Rochester, Inst Opt, Rochester, NY 14627 USA
来源：
PHYSICAL REVIEW A | 2001年 / 63卷 / 06期
关键词：
D O I：
10.1103/PhysRevA.63.063404
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
Decoherence of molecular vibrational wave packets in hot alkaline dimers due to the vibration-rotation coupling is considered. The focus is on the study of observable manifestations of the decoherence process in molecular emission tomography. Criteria are presented for control over decoherence by means of driving molecular transitions with suitably shaped ultrafast laser pulses.
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页数：9
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