Designed copper-amine complex as an efficient template for one-pot synthesis of Cu-SSZ-13 zeolite with excellent activity for selective catalytic reduction of NOx by NH3

被引:302
作者
Ren, Limin [2 ,3 ]
Zhu, Longfeng [2 ,3 ]
Yang, Chengguang [2 ,3 ]
Chen, Yanmei [4 ]
Sun, Qi [1 ]
Zhang, Haiyan [2 ,3 ]
Li, Caijin [2 ,3 ]
Nawaz, Faisal [2 ,3 ]
Meng, Xiangju [1 ]
Xiao, Feng-Shou [1 ]
机构
[1] Zhejiang Univ, Dept Chem, Hangzhou 310028, Zhejiang, Peoples R China
[2] Jilin Univ, Coll Chem, Changchun 130012, Peoples R China
[3] Jilin Univ, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Peoples R China
[4] Beijing Normal Univ, Dept Chem, Beijing 100875, Peoples R China
基金
中国国家自然科学基金;
关键词
STRUCTURE-DIRECTING AGENT; METALLOALUMINOPHOSPHATES STA-6; MOLECULAR-SIEVES; ALUMINOPHOSPHATE; METHANOL; AZAMACROCYCLE; PRODUCT; OLEFIN;
D O I
10.1039/c1cc12469b
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Low-cost copper-amine complex was rationally designed to be a novel template for one-pot synthesis of Cu-SSZ-13 zeolites. Proper confirmation and appropriate size make this complex fit well with CHA cages as an efficient template. The products exhibit superior catalytic performance on NH3-SCR reaction.
引用
收藏
页码:9789 / 9791
页数:3
相关论文
共 34 条
  • [1] Baerlocher C., 2007, ATLAS ZEOLITE FRAMEW, P96
  • [2] Nature and Location of Copper Nanospecies in Mesoporous Molecular Sieves
    Chanquia, Corina M.
    Sapag, Karim
    Rodriguez-Castellon, Enrique
    Herrero, Eduardo R.
    Eimer, Griselda A.
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2010, 114 (03) : 1481 - 1490
  • [3] Amphiphilic organosilane-directed synthesis of crystalline zeolite with tunable mesoporosity
    Choi, Minkee
    Cho, Hae Sung
    Srivastava, Rajendra
    Venkatesan, Chithravel
    Choi, Dae-Heung
    Ryoo, Ryong
    [J]. NATURE MATERIALS, 2006, 5 (09) : 718 - 723
  • [4] Stable single-unit-cell nanosheets of zeolite MFI as active and long-lived catalysts
    Choi, Minkee
    Na, Kyungsu
    Kim, Jeongnam
    Sakamoto, Yasuhiro
    Terasaki, Osamu
    Ryoo, Ryong
    [J]. NATURE, 2009, 461 (7261) : 246 - U120
  • [5] Ionic liquids and eutectic mixtures as solvent and template in synthesis of zeolite analogues
    Cooper, ER
    Andrews, CD
    Wheatley, PS
    Webb, PB
    Wormald, P
    Morris, RE
    [J]. NATURE, 2004, 430 (7003) : 1012 - 1016
  • [6] Supramolecular self-assembled molecules as organic directing agent for synthesis of zeolites
    Corma, A
    Rey, F
    Rius, J
    Sabater, MJ
    Valencia, S
    [J]. NATURE, 2004, 431 (7006) : 287 - 290
  • [7] INORGANIC SOLID ACIDS AND THEIR USE IN ACID-CATALYZED HYDROCARBON REACTIONS
    CORMA, A
    [J]. CHEMICAL REVIEWS, 1995, 95 (03) : 559 - 614
  • [8] The hydrothermal synthesis of zeolites: History and development from the earliest days to the present time
    Cundy, CS
    Cox, PA
    [J]. CHEMICAL REVIEWS, 2003, 103 (03) : 663 - 701
  • [9] Ordered porous materials for emerging applications
    Davis, ME
    [J]. NATURE, 2002, 417 (6891) : 813 - 821
  • [10] SYNTHESIS OF NEW SILICA-RICH CUBIC AND HEXAGONAL FAUJASITES USING CROWN-ETHER-BASED SUPRAMOLECULES AS TEMPLATES
    DELPRATO, F
    DELMOTTE, L
    GUTH, JL
    HUVE, L
    [J]. ZEOLITES, 1990, 10 (06): : 546 - 552