Tuning of dielectric properties of SrTiO3 in the terahertz range

被引:25
作者
Skoromets, V. [1 ]
Kadlec, F. [1 ]
Kadlec, C. [1 ]
Nemec, H. [1 ]
Rychetsky, I. [1 ]
Panaitov, G. [2 ]
Mueller, V. [3 ]
Fattakhova-Rohlfing, D. [3 ]
Moch, P. [4 ]
Kuzel, P. [1 ]
机构
[1] Acad Sci Czech Republic, Inst Phys, CZ-18221 Prague 8, Czech Republic
[2] Forschungszentrum Julich, Inst Bio & Nanosyst, D-52425 Julich, Germany
[3] Univ Munich LMU, Dept Chem & Biochem, D-81377 Munich, Germany
[4] Univ Paris 13, LSPM, CNRS, UPR 3407, F-93430 Villetaneuse, France
来源
PHYSICAL REVIEW B | 2011年 / 84卷 / 17期
关键词
STRONTIUM-TITANATE; RAMAN SCATTERING; SPECTROSCOPY;
D O I
10.1103/PhysRevB.84.174121
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Tuning of the dielectric permittivity spectra of strontium titanate (SrTiO3) single crystals in an external electric field is investigated between 90 and 300 K by means of terahertz time-domain spectroscopy. Application of the electric bias leads to an appreciable tuning of the permittivity observed up to room temperature both in the parallel and perpendicular directions to the bias field. The observed behavior is interpreted in terms of soft-mode hardening due to the anharmonic character of its potential. No additional low-frequency relaxation mode was observed. A weak temperature dependence of the anharmonic coefficients was found in agreement with previously published low-temperature data.
引用
收藏
页数:10
相关论文
共 24 条
[1]   Strain tensor effects on SrTiO3 incipient ferroelectric phase transition [J].
Chang, Wontae ;
Bellotti, Jeffrey A. ;
Kirchoefer, Steven W. ;
Pond, Jeffrey M. .
JOURNAL OF ELECTROCERAMICS, 2006, 17 (2-4) :487-494
[2]   DIELECTRIC-PROPERTIES OF SPUTTERED SRTIO3 FILMS [J].
CHRISTEN, HM ;
MANNHART, J ;
WILLIAMS, EJ ;
GERBER, C .
PHYSICAL REVIEW B, 1994, 49 (17) :12095-12104
[3]   Scaling behaviour of strontium titanate [J].
Dec, J ;
Kleemann, W ;
Westwanski, B .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1999, 11 (32) :L379-L384
[4]   A reliable method for extraction of material parameters in terahertz time-domain spectroscopy [J].
Duvillaret, L ;
Garet, F ;
Coutaz, JL .
IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, 1996, 2 (03) :739-746
[5]   Orientation and direct current field dependent dielectric properties of bulk single crystal SrTiO3 at microwave frequencies [J].
Eriksson, A ;
Deleniv, A ;
Gevorgian, S .
JOURNAL OF APPLIED PHYSICS, 2003, 93 (05) :2848-2854
[6]   ELECTRIC-FIELD-INDUCED RAMAN SCATTERING IN SRTIO3 AND KTAO3 [J].
FLEURY, PA ;
WORLOCK, JM .
PHYSICAL REVIEW, 1968, 174 (02) :613-&
[7]   Room-temperature ferroelectricity in strained SrTiO3 [J].
Haeni, JH ;
Irvin, P ;
Chang, W ;
Uecker, R ;
Reiche, P ;
Li, YL ;
Choudhury, S ;
Tian, W ;
Hawley, ME ;
Craigo, B ;
Tagantsev, AK ;
Pan, XQ ;
Streiffer, SK ;
Chen, LQ ;
Kirchoefer, SW ;
Levy, J ;
Schlom, DG .
NATURE, 2004, 430 (7001) :758-761
[8]  
Hecht F., Freefem++
[9]   ELECTRIC-FIELD-DEPENDENT DIELECTRIC-CONSTANT AND NONLINEAR SUSCEPTIBILITY IN SRTIO3 [J].
HEMBERGER, J ;
LUNKENHEIMER, P ;
VIANA, R ;
BOHMER, R ;
LOIDL, A .
PHYSICAL REVIEW B, 1995, 52 (18) :13159-13162
[10]   Coexistence of the Phonon and Relaxation Soft Modes in the Terahertz Dielectric Response of Tetragonal BaTiO3 [J].
Hlinka, J. ;
Ostapchuk, T. ;
Nuzhnyy, D. ;
Petzelt, J. ;
Kuzel, P. ;
Kadlec, C. ;
Vanek, P. ;
Ponomareva, I. ;
Bellaiche, L. .
PHYSICAL REVIEW LETTERS, 2008, 101 (16)