Direct observation of mode selective electron-phonon coupling in suspended carbon nanotubes

被引:59
作者
Bushmaker, Adam W. [1 ]
Deshpande, Vikram V. [2 ]
Bockrath, Marc W. [2 ]
Cronin, Stephen B. [1 ]
机构
[1] Univ So Calif, Dept Elect Engn, Los Angeles, CA 90089 USA
[2] CALTECH, Pasadena, CA 91125 USA
关键词
D O I
10.1021/nl071840f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Raman spectra of individual pristine suspended single-walled carbon nanotubes are observed under high electrical bias. The LO and TO modes of the G band behave differently with respect to voltage bias, indicating preferential electron-phonon coupling and nonequilibrium phonon populations, which cause negative differential conductance in suspended devices. By correlating the electron resistivity to the optically measured phonon population, the data are fit using a Landauer model to determine the key scattering parameters.
引用
收藏
页码:3618 / 3622
页数:5
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