Alkylative/arylative carboxylation of unsaturated hydrocarbons utilizing CO2 as C1 synthon: An update

被引:7
作者
Cao, Yan [1 ]
Dhahad, Hayder A. [2 ]
Hussen, Hasanen M. [2 ]
Anqi, Ali E. [3 ]
Farouk, Naeim [4 ,5 ]
Issakhov, Alibek [6 ,7 ]
Heravi, Mohammad Reza Poor [8 ]
机构
[1] Xian Technol Univ, Sch Mech Engn, Xian 710021, Peoples R China
[2] Univ Technol Baghdad, Mech Engn Dept, Baghdad, Iraq
[3] King Khalid Univ, Dept Mech Engn, Coll Engn, Abha 61421, Saudi Arabia
[4] Prince Sattam Bin Abdulaziz Univ, Mech Engn Dept, Coll Engn, Alkharj 16273, Saudi Arabia
[5] Red Sea Univ Port Sudan, Mech Engn Dept, Fac Engn, Port Sudan, Sudan
[6] Al Farabi Kazakh Natl Univ, Dept Math & Comp Modelling, Alma Ata 050040, Kazakhstan
[7] Kazakh British Tech Univ, Dept Math & Cybernet, Alma Ata 050000, Kazakhstan
[8] Payame Noor Univ, Dept Chem, Tehran, Iran
关键词
Carbon dioxide; Difunctionalization; Carbocarboxylation; Unsaturated hydrocarbons; Carboxylic acids; COPPER-CATALYZED CARBOXYLATION; ENVIRONMENTALLY BENIGN ACCESS; CARBON-DIOXIDE; CHEMICAL FIXATION; STRAIGHTFORWARD ROUTE; DIALKYLZINC REAGENTS; EFFICIENT SYNTHESIS; GREEN ROUTE; PHOTOREDOX; ALKENES;
D O I
10.1016/j.jcou.2021.101664
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The difunctionalization of unsaturated hydrocarbons, the incorporation of two functional groups onto an unsaturated carbon-carbon bonds, is one of the most active and popular topics in modern organic chemistry due to its significance in the rapid and highly atom economical synthesis of complex molecules from simple starting materials within a single click. Among various difunctionalization reactions, difunctionalizing carboxylations utilizing CO2 as a renewable and environmental friendly C1 feedstock has attracted more and more attention in recent years. In this regard, several interesting strategies have been developed in the last two decades for the preparation of branched carboxylic acids and their derivatives through the alkylative/arylative carboxylation of the corresponding unsaturated hydrocarbons using CO2 as a carboxyl source. Thus, it is an appropriate time to summarize those advances. The purpose of this Mini-Review is to focus on the most important advances and developments on the attractive research field with particular emphasis on the mechanistic features of the reaction pathways. Notably, we have organized this review based on the type of bond where the CO2 insertion occurs.
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页数:11
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